Highly anisotropic magnetism in the vanadium-based kagome metal TbV6Sn6

Abstract

RV6Sn6 (R=rare earth) compounds are appealing materials platforms for exploring the interplay between R-site magnetism and nontrivial band topology associated with the nonmagnetic vanadium-based kagome network. Here we present the synthesis and characterization of the kagome metal TbV6Sn6 via single-crystal x-ray diffraction, magnetization, transport, and heat capacity measurements. Magnetization measurements reveal strong, uniaxial magnetic anisotropy rooted in the alignment of Tb3Å moments in the interplane direction below 4.3(2) K. TbV6Sn6 exhibits multiband transport behavior with high mobilities of charge carriers, and our measurements suggest TbV6Sn6 is a promising candidate for hosting Chern gaps driven via the interplay between Tb-site magnetic order and the band topology of the V-site kagome network.

References in corpus (18)

• CsV${}_3$Sb${}_5$: a ${\mathbb{Z}}_2$ topological kagome metal with a superconducting ground state
• Discovery of unconventional chiral charge order in kagome superconductor KV3Sb5
• Cascade of correlated electron states in a kagome superconductor CsV3Sb5
• Discovery of a quantum limit Chern magnet TbMn6Sn6
• Superconductivity in the ${\mathbb{Z}}_2$ kagome metal KV${}_3$Sb${}_5$
• Superconductivity and normal-state properties of kagome metal RbV3Sb5 single crystals
• Electrical Manipulation of a Topological Antiferromagnetic State
• Discovery of charge density wave in a correlated kagome lattice antiferromagnet
• Unified explanation of the Kadowaki-Woods ratio in strongly correlated materials
• Realizing Kagome Band Structure in Two-Dimensional Kagome Surface States of $R{V}_{6}S{n}_6$ ($R$=Gd,Ho)
• Study of the electronic properties of topological kagome metals YV${}_6$Sn${}_6$ and GdV${}_6$Sn${}_6$
• Large anomalous Hall effect in the kagome ferromagnet LiMn${}_6$Sn${}_6$
• Topological charge-entropy scaling in kagome Chern magnet TbMn${}_6$Sn${}_6$
• Anomalous Hall Effect in Kagome Ferrimagnet GdMn${}_6$Sn${}_6$
• Chiral properties of the zero-field spiral state and field-induced magnetic phases of the itinerant kagome metal YMn${}_6$Sn${}_6$
• GdV6Sn6: a Multi-carrier Metal with Non-magnetic 3d-electron Kagome Bands and 4f-electron Magnetism
• Quantum critical behaviour of the plateau-insulator transition in the quantum Hall regime
• Evolution of the Chern Gap in Chern Magnet HoMn${}_6$Sn${}_{6-x}$Ge${}_x$

Cited by in corpus (30)

• AV${}_3$Sb${}_5$ Kagome Superconductors: Progress and Future Directions
• Abundant lattice instability in kagome metal ScV${}_6$Sn${}_6$
• Flat band separation and robust spin-Berry curvature in bilayer kagome metals
• Quantum Interactions in Topological R166 Kagome Magnet
• Evolution of highly anisotropic magnetism in the titanium-based kagome metals LnTi${}_3$Bi${}_4$ (Ln: La...Gd${}^{3+}$, Eu${}^{2+}$, Yb${}^{2+}$)
• Nanoscale visualization and spectral fingerprints of the charge order in ScV6Sn6 distinct from other kagome metals
• Frustrated charge order and cooperative distortions in ScV6Sn6
• Tiny Sc allows the chains to rattle: Impact of Lu and Y doping on the charge density wave in ScV${}_6$Sn${}_6$
• Dynamics and Resilience of the Charge Density Wave in a bilayer kagome metal
• Triangular Kondo lattice in $\mathrm{Yb}{\mathrm{V}}_6\mathrm{S}{\mathrm{n}}_6$ and its quantum critical behaviors in magnetic field
• Universal sublinear resistivity in vanadium kagome materials hosting charge density waves
• Stability frontiers in the AM${}_6$X${}_6$ kagome metals: The LnNb${}_6$Sn${}_6$ (Ln:Ce-Lu,Y) family and density-wave transition in LuNb${}_6$Sn${}_6$
• Anisotropic magnetism and band evolution induced by ferromagnetic phase transition in titanium-based kagome ferromagnet SmTi3Bi4
• YbV${}_3$Sb${}_4$ and EuV${}_3$Sb${}_4$, vanadium-based kagome metals with Yb${}^{2+}$ and Eu${}^{2+}$ zig-zag chains
• Colossal orbital Zeeman effect driven by tunable spin-Berry curvature in a kagome metal
• Toward a first-principles theory of rare-earth ions in crystals
• Kagome metals
• Intricate magnetic landscape in antiferromagnetic kagome metal TbTi${}_3$Bi${}_4$ and interplay with Ln${}_{2-x}$Ti${}_{6+x}$Bi${}_9$ (Ln: Tb-Lu) shurikagome metals
• Electronic band structures of topological kagome materials
• Incommensurate Magnetic Order in the ${\mathbb{Z}}_2$ Kagome Metal GdV${}_6$Sn${}_6$
• Ground-state magnetic structures of topological kagome metals RV${}_6$Sn${}_6$ (R = Tb, Dy, Ho, Er)
• Kagome surface states and weak electronic correlation in vanadium-kagome metals
• Competing Lattice Instability and Magnetism on the Surface of Kagome Metals
• Kagome Metal GdNb${}_6$Sn${}_6$: A 4d Playground for Topological Magnetism and Electron Correlations
• The electronic structure of intertwined kagome, honeycomb, and triangular sublattices of the intermetallics MCo${}_2$Al${}_9$
• Strongly Entangled Kondo and Kagome Lattices and the Emergent Magnetic Ground State in Heavy-Fermion Kagome Metal YbV${}_6$Sn${}_6$
• Magnetic order and physical properties of the Kagome metal UNb${}_6$Sn${}_6$
• Magnetic properties of van der Waals layered single crystals DyOBr and SmOCl
• Nature of quantum criticality in the Ising ferromagnet TbV${}_6$Sn${}_6$
• Structural modulation, physical properties, and electronic band structure of the kagome metal UCr${}_6$Ge${}_6$