Pseudospin-lattice coupling and electric control of the square-lattice iridate Sr2IrO4

Abstract

$\mathrm{S}{\mathrm{r}}_2\mathrm{Ir}{\mathrm{O}}_4$ is an archetypal spin-orbit-coupled Mott insulator and has been extensively studied in part because of a wide range of predicted novel states. Limited experimental characterization of these states thus far brings to light the extraordinary susceptibility of the physical properties to the lattice, particularly, the Ir-O-Ir bond angle. Here, we report a newly observed microscopic rotation of the IrO${}_6$ octahedra below 50~K measured by single crystal neutron diffraction. This sharp lattice anomaly provides keys to understanding the anomalous low-temperature physics and a direct confirmation of a crucial role that the Ir-O-Ir bond angle plays in determining the ground state. Indeed, as also demonstrated in this study, applied electric current readily weakens the antiferromagnetic order via the straightening of the Ir-O-Ir bond angle, highlighting that even slight change in the local structure can disproportionately affect the physical properties in the spin-orbit-coupled system.

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Cited by in corpus (4)

• Quest for New Quantum States via Field-Editing Technology
• Evolution of electronic and magnetic properties of Sr${}_2$IrO${}_4$ under strain
• Quantum Criticality in a Layered Iridate
• Fortuitous partners of antiferromagnetic and Mott states in spin-orbit-coupled Sr2IrO4: A study of Sr2Ir1-xMxO4 (M=Fe or Co)