Creation of vibrationally-excited ultralong-range Rydberg molecules in polarized and unpolarized cold gases of ${}^{87}$Sr

Abstract

Photoexcitation rates for creation of ultralong-range Rydberg molecules (ULRM) with 31$\lesssim n\lesssim 41$ in both ground and excited vibrational levels in cold ($T\sim 900$~nK) gases of polarized and unpolarized ${}^{87}$Sr are presented. The measured production rates of the $\nu =0,1$ and 2 vibrational levels reveal rather different $n$ dependences which are analyzed by evaluating the Franck-Condon factors associated with excitation of the different vibrational levels and molecular rotational states. In particular, for gases of spin-polarized fermions, only Rydberg dimers with odd rotational quantum numbers are excited due to the requirement that their wavefunctions be anti-symmetric with respect to exchange. The data also demonstrate that measurements of the formation of vibrationally-excited $\nu =1$ molecules can furnish a probe of pair correlations over intermediate length scales extending from $\sim 20$~nm to greater than 250~nm.

arXiv comment18 pages, 9 figures

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• Long-range Rydberg molecule Rb${}_2$: Two-electron \textit{R}-matrix calculations at intermediate internuclear distances