Electric-dipole active two-magnon excitation in {\textit{ab}} spiral spin phase of a ferroelectric magnet GdTbMnO
arXiv:0811.4098 · doi:10.1143/JPSJ.77.123704
Abstract
A broad continuum-like spin excitation (1--10 meV) with a peak structure around 2.4 meV has been observed in the ferroelectric spiral spin phase of GdTbMnO by using terahertz (THz) time-domain spectroscopy. Based on a complete set of light-polarization measurements, we identify the spin excitation active for the light vector only along the a-axis, which grows in intensity with lowering temperature even from above the magnetic ordering temperature but disappears upon the transition to the -type antiferromagnetic phase. Such an electric-dipole active spin excitation as observed at THz frequencies can be ascribed to the two-magnon excitation in terms of the unique polarization selection rule in a variety of the magnetically ordered phases.
11 pages including 3 figures
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Cited by in corpus (6)
- Electrodynamics of Correlated Electron Materials
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- Terahertz time-domain spectroscopy of electromagnons in multiferroic perovskite manganites
- Magnetic and magnetoelectric excitations in TbMnO
- Theoretically predicted picosecond optical switching of spin chirality in multiferroics
- Modeling and Physics of Multiferroic Perovskite Manganites