Relaxations as key to the magnetocapacitive effects in the perovskite manganites

Abstract

We present a detailed dielectric study of the relaxation effects that occur in several perovskite rare-earth manganites, including the multiferroics TbMnO3 and DyMnO3. We demonstrate that the strong magnetocapacitive effects, observed for electrical fields E||c, are nearly completely governed by magnetic-state induced changes of the relaxation parameters. The multiferroic materials, which undergo a transition into a spiral magnetic state, show qualitatively different relaxation behavior than those compounds transferring into an A-type antiferromagnetic state. We ascribe the relaxations in both cases to the off-center motion of the manganese ions, which in the multiferroic systems also leads to the ferroelectric ordering.

arXiv comment4 pages; 4 figures; final version, revised according to suggestions of referees

References in corpus (13)

• Spin current and magneto-electric effect in non-collinear magnets
• Ferroelectricity in spiral magnets
• Role of the Dzyaloshinskii-Moriya interaction in multiferroic perovskites
• Materials with Colossal Dielectric Constant: Do They Exist?
• Magnetic inversion symmetry breaking and ferroelectricity in TbMnO3
• Distorted Perovskite with e_g^1 Configuration as a Frustrated Spin System
• Possible evidence for electromagnons in multiferroic manganites
• Collinear-to-Spiral Spin Transformation without Changing Modulation Wavelength upon Ferroelectric Transition in Tb1-xDyxMnO3
• Spin-Orbit Coupling and Ion Displacements in Multiferroic TbMnO3
• First-principles study of improper ferroelectricity in TbMnO3
• The multiferroic phases of (Eu:Y)MnO3
• Dynamics of Multiferroic Domain Wall in Spin-Cycloidal Ferroelectric DyMnO${}_3$
• Magnetic-Field and External-Pressure Control of Ferroelectricity in Multiferroic Manganites

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