Magnetoelectric Effect and Spontaneous Polarization in HoFe(BO) and HoNdFe(BO)
arXiv:0906.1227 · doi:10.1103/PhysRevB.80.104424
Abstract
The thermodynamic, magnetic, dielectric, and magnetoelectric properties of HoFe(BO) and HoNdFe(BO) are investigated. Both compounds show a second order Neél transition above 30 K and a first order spin reorientation transition below 10 K. HoFe(BO) develops a spontaneous electrical polarization below the Neél temperature (T) which is diminished in external magnetic fields. No magnetoelectric effect could be observed in HoFe(BO). In contrast, the solid solution HoNdFe(BO) exhibits both, a spontaneous polarization below T and a magnetoelectric effect at higher fields that extends to high temperatures. The superposition of spontaneous polarization, induced by the internal magnetic field in the ordered state, and the magnetoelectric polarizations due to the external field results in a complex behavior of the total polarization measured as a function of temperature and field.
12 pages, 15 figures
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