Magnetic Field-Induced Condensation of Triplons in Han Purple Pigment BaCuSi${}_2$O${}_6$

Abstract

Besides being an ancient pigment, BaCuSi${}_2$O${}_6$ is a quasi-2D magnetic insulator with a gapped spin dimer ground state. The application of strong magnetic fields closes this gap creating a gas of bosonic spin triplet excitations called triplons. The topology of the spin lattice makes BaCuSi${}_2$O${}_6$ an ideal candidate for studying the Bose-Einstein condensation of triplons as a function of the external magnetic field, which acts as a chemical potential. In agreement with quantum Monte Carlo numerical simulations, we observe a distinct lambda-anomaly in the specific heat together with a maximum in the magnetic susceptibility upon cooling down to liquid Helium temperatures.

published on August 20, 2004

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