Spin-density wave and superconductivity in La${}_4$Ni${}_3$O${}_{10}$ under ambient pressure

Abstract

We investigate the spin-density wave (SDW) behavior and the potential for superconductivity (SC) in La${}_4$Ni${}_3$O${}_{10}$ under ambient pressure using a multi-orbital random-phase approximation (RPA). Starting with a twelve-orbital tight-binding model derived from density functional theory (DFT) calculations, we explore the influence of Hubbard interactions on SDW formation. Our analysis reveals a stripe-like SDW characterized by an incommensurate wave vector, $Q\approx (\pm 0.7\pi ,0)$, suggesting a possible density wave instability in agreement with recent experiments. This configuration is driven by nesting of outer-layer Ni $d_{z^2}$ orbitals and exhibits interlayer antiferromagnetic ordering between the top and bottom NiO layers, with the middle layer serving as a node. We demonstrate that the Hund's coupling $J_H$ is the primary driver of the observed SDW. While superconductivity is absent in the undoped system under ambient pressure, it becomes attainable with appropriate hole doping ($\delta =-0.4$), resulting in a SC gap structure similar to the high-pressure phase. Our study identifies the specific conditions for realizing the ambient pressure stripe density wave: $J_H>0.16U$. Additionally, when doping leads to sufficient nesting at (0,0), the system's magnetic fluctuations transition into a stable Neel-type antiferromagnetic state, analogous to the high-pressure case.

6 pages, 7 figures

References in corpus (88)

• Restoring the density-gradient expansion for exchange in solids and surfaces
• Generalized gradient approximation for solids and their surfaces
• Unconventional pairing originating from disconnected Fermi surfaces in superconducting LaFeAsO${}_{1-x}$F${}_x$}
• Near-degeneracy of several pairing channels in multiorbital models for the Fe-pnictides
• Superconductivity near 80 Kelvin in single crystals of La3Ni2O7 under pressure
• Funtional Renormalization Group Study of the Pairing Symmetry and Pairing Mechanism of the FeAs Based High Temperature Superconductors
• High-temperature superconductivity with zero-resistance and strange metal behavior in La${}_3$Ni${}_2$O${}_{7-\delta }$
• Bilayer two-orbital model of La${}_3$Ni${}_2$O${}_7$ under pressure
• Superconductivity in pressurized trilayer La${}_4$Ni${}_3$O${}_{10-\delta }$ single crystals
• Visualization of Oxygen Vacancies and Self-doped Ligand Holes in La3Ni2O7-δ
• Possible $S_{\pm }$-wave superconductivity in La${}_3$Ni${}_2$O${}_7$
• The s${}^{\pm }$-Wave Pairing and the Destructive Role of Apical-Oxygen Deficiencies in La${}_3$Ni${}_2$O${}_7$ Under Pressure
• Possible high $T_c$ Superconductivity in La${}_3$Ni${}_2$O${}_7$ under High Pressure through Manifestation of a Nearly-Half-Filled Bilayer Hubbard Model
• Electronic correlations and superconducting instability in La${}_3$Ni${}_2$O${}_7$ under high pressure
• Interlayer Coupling Driven High-Temperature Superconductivity in La${}_3$Ni${}_2$O${}_7$ Under Pressure
• Correlated electronic structure of La${}_3$Ni${}_2$O${}_7$ under pressure
• Orbital-Dependent Electron Correlation in Double-Layer Nickelate La3Ni2O7
• Bilayer $t$-$J$-$J_{\perp }$ Model and Magnetically Mediated Pairing in the Pressurized Nickelate La${}_3$Ni${}_2$O${}_7$
• Evidence for charge and spin order in single crystals of La${}_3$Ni${}_2$O${}_7$ and La${}_3$Ni${}_2$O${}_6$
• Effective bi-layer model Hamiltonian and density-matrix renormalization group study for the high-Tc superconductivity in La${}_3$Ni${}_2$O${}_7$ under high pressure
• Electronic structure, dimer physics, orbital-selective behavior, and magnetic tendencies in the bilayer nickelate superconductor La${}_3$Ni${}_2$O${}_7$ under pressure
• Pressure-induced superconductivity in polycrystalline La3Ni2O7
• Structural phase transition, $s_{\pm }$-wave pairing and magnetic stripe order in the bilayered nickelate superconductor La${}_3$Ni${}_2$O${}_7$ under pressure
• Signature of superconductivity in pressurized La${}_4$Ni${}_3$O${}_{10}$
• Character of the "normal state" of the nickelate superconductors
• Electronic and magnetic excitations in La${}_3$Ni${}_2$O${}_7$
• High-$T_c$ superconductivity by mobilizing local spin singlets and possible route to higher $T_c$ in pressurized La${}_3$Ni${}_2$O${}_7$
• High Temperature Superconductivity in La${}_3$Ni${}_2$O${}_7$
• Theoretical analysis on the possibility of superconductivity in a trilayer Ruddlesden-Popper nickelate La${}_4$Ni${}_3$O${}_{10}$ under pressure and its experimental examination: comparison with La${}_3$Ni${}_2$O${}_7$
• Electronic correlations and partial gap in the bilayer nickelate La${}_3$Ni${}_2$O${}_7$
• Flat bands promoted by Hund's rule coupling in the candidate double-layer high-temperature superconductor La${}_3$Ni${}_2$O${}_7$
• Correlated electronic structure, orbital-selective behavior, and magnetic correlations in double-layer La${}_3$Ni${}_2$O${}_7$ under pressure
• Structure responsible for the superconducting state in La3Ni2O7 at high pressure and low temperature conditions
• Charge Transfer and Zhang-Rice Singlet Bands in the Nickelate Superconductor $\mathrm{L}{\mathrm{a}}_3\mathrm{N}{\mathrm{i}}_2{\mathrm{O}}_7$ under Pressure
• Polymorphism in Ruddlesden-Popper $L{a}_{3}N{i}_2{O}_7$: Discovery of a Hidden Phase with Distinctive Layer Stacking
• Pairing symmetry in a two-orbital Hubbard model on a square lattice
• Correlation Effects and Concomitant Two-Orbital $s_{\pm }$-Wave Superconductivity in La${}_3$Ni${}_2$O${}_7$ under High Pressure
• Trends in electronic structures and $s_{\pm }$-wave pairing for the rare-earth series in bilayer nickelate superconductor $R_3$Ni${}_2$O${}_7$
• Electron correlations and superconductivity in La${}_3$Ni${}_2$O${}_7$ under pressure tuning
• Effects of Pressure and Doping on Ruddlesden-Popper phases Lan+1NinO3n+1
• High-T${}_C$ superconductivity in $\mathrm{L}{\mathrm{a}}_3\mathrm{N}{\mathrm{i}}_2{\mathrm{O}}_7$ based on the bilayer two-orbital t-J model
• Pressure Driven Fractionalization of Ionic Spins Results in Cupratelike High-$T_c$ Superconductivity in La${}_3$Ni${}_2$O${}_7$
• Superconductivity in nickelate and cuprate superconductors with strong bilayer coupling
• Impurity and vortex States in the bilayer high-temperature superconductor ${\mathrm{La}}_3{\mathrm{Ni}}_2{\mathrm{O}}_7$
• Neutron Scattering Studies on the High-$T_c$ Superconductor La${}_3$Ni${}_2$O${}_{7-\delta }$ at Ambient Pressure
• Pressure-enhanced spin-density-wave transition in double-layer nickelate $L{a}_{3}N{i}_2{O}_{7-\delta }$
• Structural transitions, octahedral rotations, and electronic properties of $A_3$Ni${}_2$O${}_7$ rare-earth nickelates under high pressure
• Competing d${}_{xy}$ and s${}_{\pm }$ Pairing Symmetries in Superconducting La${}_3$Ni${}_2$O${}_7$ emerge from LDA+FLEX Calculations
• Structural transition, electric transport, and electronic structures in the compressed trilayer nickelate La4Ni3O10
• Multiband Metallic Ground State in Multilayered Nickelates La${}_3$Ni${}_2$O${}_7$ and La${}_4$Ni${}_3$O${}_{10}$ Probed by ${}^{139}$La-NMR at Ambient Pressure
• Quenched pair breaking by interlayer correlations as a key to superconductivity in La${}_3$Ni${}_2$O${}_7$
• Pressure-enhanced splitting of density wave transitions in La${}_3$Ni${}_2$O${}_{7-\delta }$
• Pair correlations in the two-orbital Hubbard ladder: Implications on superconductivity in the bilayer nickelate La${}_3$Ni${}_2$O${}_7$
• Sensitive dependence of pairing symmetry on Ni-$e_g$ crystal field splitting in the nickelate superconductor La${}_3$Ni${}_2$O${}_7$
• Hund electronic correlation in La${}_3$Ni${}_2$O${}_7$ under high pressure
• Effective model and $s_{\pm }$-wave superconductivity in trilayer nickelate La${}_4$Ni${}_3$O${}_{10}$
• Superconducting state of Sr${}_2$RuO${}_4$ in the presence of longer-range Coulomb interactions
• Strong Pairing Originated from an Emergent ${\mathbb{Z}}_2$ Berry Phase in La${}_3$Ni${}_2$O${}_7$
• Prediction of $s^{\pm }$-wave superconductivity enhanced by electronic doping in trilayer nickelates La${}_4$Ni${}_3$O${}_{10}$ under pressure
• Superconductivity from repulsive interactions on the kagome lattice
• Structural routes to stabilise superconducting La${}_3$Ni${}_2$O${}_7$ at ambient pressure
• Theory of magnetic excitations in multilayer nickelate superconductor La${}_3$Ni${}_2$O${}_7$
• The electronic and magnetic structures of bilayer La${}_3$Ni${}_2$O${}_7$ at ambient pressure
• Electronic structure, magnetic correlations, and superconducting pairing in the reduced Ruddlesden-Popper bilayer La${}_3$Ni${}_2$O${}_6$ under pressure: different role of $d_{3z^2-r^2}$ orbital compared with La${}_3$Ni${}_2$O${}_7$
• Trilayer multi-orbital models of $\mathrm{L}{\mathrm{a}}_4\mathrm{N}{\mathrm{i}}_3{\mathrm{O}}_{10}$
• Non-Fermi Liquid and Hund Correlation in La${}_4$Ni${}_3$O${}_{10}$ under High Pressure
• Electronic Correlation and Pseudogap-like Behavior of High-Temperature Superconductor La3Ni2O7
• Theory of Pressure Dependence of Superconductivity in Bilayer Nickelate La${}_3$Ni${}_2$O${}_7$
• Effect of Rare-earth Element Substitution in Superconducting R${}_3$Ni${}_2$O${}_7$ Under Pressure
• Charge and spin instabilities in superconducting La${}_3$Ni${}_2$O${}_7$
• Density-wave-like gap evolution in La${}_3$Ni${}_2$O${}_7$ under high pressure revealed by ultrafast optical spectroscopy
• Ultrafast Dynamics of Bilayer and Trilayer Nickelate Superconductors
• Optical properties and electronic correlations in La${}_3$Ni${}_2$O${}_7$ bilayer nickelates under high pressure
• Antiferromagnetic Ground State, Charge Density Waves and Oxygen Vacancies Induced Metal-Insulator Transition in Pressurized La${}_3$Ni${}_2$O${}_7$
• Signature of Superconductivity in Pressurized Trilayer-nickelate Pr${}_4$Ni${}_3$O${}_{10-\delta }$
• The $s^{\pm }$-Wave Superconductivity in the Pressurized La${}_4$Ni${}_3$O${}_{10}$
• Electronic structure and magnetic correlations in trilayer nickelate superconductor La${}_4$Ni${}_3$O${}_{10}$ under pressure
• Electronic properties of nickelate superconductor R3Ni2O7 with oxygen vacancies
• Effective model and electron correlations in trilayer nickelate superconductor La${}_4$Ni${}_3$O${}_{10}$
• Origin of the density wave instability in trilayer nickelate La${}_4$Ni${}_3$O${}_{10}$ revealed by optical and ultrafast spectroscopy
• Assessing the formation of spin and charge stripes in La${}_3$Ni${}_2$O${}_7$ from first-principles
• High-pressure crystal growth and investigation of the metal-to-metal transition of Ruddlesden-Popper trilayer nickelates La${}_4$Ni${}_3$O${}_{10}$
• Magnetic phase diagram of a two-orbital model for bilayer nickelates varying doping
• Interlayer Pairing Induced Partially Gapped Fermi Surface in Trilayer La${}_4$Ni${}_3$O${}_{10}$ Superconductors
• Decomposition of multilayer superconductivity with interlayer pairing
• Non-Fermi liquid and antiferromagnetic correlations with hole doping in the bilayer two-orbital Hubbard model of La${}_3$Ni${}_2$O${}_7$ at zero temperature
• Lifshitz transition enhanced triplet $p_z$-wave superconductivity in hydrogen doped KCr${}_3$As${}_3$
• Correlation Effects in a Simplified Bilayer Two-Orbital Hubbard Model at Half Filling

Cited by in corpus (6)

• General trends of electronic structures, superconducting pairing, and magnetic correlations in the Ruddlesden-Popper nickelate $m$-layered superconductors La${}_{m+1}$Ni${}_m$O${}_{3m+1}$
• Orbital-Selective Quasiparticle Depletion across the Density Wave Transition in Trilayer Nickelate La${}_4$Ni${}_3$O${}_{10}$
• Electronic layer decoupling driven by density-wave order in La${}_4$Ni${}_3$O${}_{10}$
• Multiorbital character of the density wave in trilayer nickelate superconductors
• Intertwined Charge and Spin Density Waves in Trilayer Nickelate La${}_4$Ni${}_3$O${}_{10}$ Revealed by ${}^{139}$La NQR
• Magnetically Mediated Cross-Layer Pairing in Pressurized Trilayer Nickelate La${}_4$Ni${}_3$O${}_{10}$