Orbital-Selective Quasiparticle Depletion across the Density Wave Transition in Trilayer Nickelate La${}_4$Ni${}_3$O${}_{10}$

Abstract

We investigate the evolution of polarized electronic Raman response in trilayer nickelate La${}_4$Ni${}_3$O${}_{10}$, uncovering a systematic reduction of the incoherent electron continuum across the density wave transition in the $A_{1g}$ and $B_{1g}$ representations. Analysis based on the Fermi surface band curvatures points to quasiparticle coherence in momentum positions with dominant $d_{x^2-y^2}$ orbital character. Our findings establish the symmetry channels and the active role of $d_{x^2-y^2}$ orbitals involved in the density wave formation, offering important insight into the electronic and magnetic correlations in the nickelate.

Revised version accepted in Phys. Rev. Lett. New Table, Supplemental figures, and additional descriptions have been included. (Main text) 13 pages, 4 figures, 1 table. (Supplemental materials) 11 pages, 7 figures

References in corpus (32)

• Superconductivity near 80 Kelvin in single crystals of La3Ni2O7 under pressure
• Inelastic Light Scattering From Correlated Electrons
• Superconductivity in pressurized trilayer La${}_4$Ni${}_3$O${}_{10-\delta }$ single crystals
• Possible $S_{\pm }$-wave superconductivity in La${}_3$Ni${}_2$O${}_7$
• The s${}^{\pm }$-Wave Pairing and the Destructive Role of Apical-Oxygen Deficiencies in La${}_3$Ni${}_2$O${}_7$ Under Pressure
• Electronic correlations and superconducting instability in La${}_3$Ni${}_2$O${}_7$ under high pressure
• Possible high $T_c$ Superconductivity in La${}_3$Ni${}_2$O${}_7$ under High Pressure through Manifestation of a Nearly-Half-Filled Bilayer Hubbard Model
• Interlayer Coupling Driven High-Temperature Superconductivity in La${}_3$Ni${}_2$O${}_7$ Under Pressure
• Orbital-Dependent Electron Correlation in Double-Layer Nickelate La3Ni2O7
• Bilayer $t$-$J$-$J_{\perp }$ Model and Magnetically Mediated Pairing in the Pressurized Nickelate La${}_3$Ni${}_2$O${}_7$
• Pressure-induced superconductivity in polycrystalline La3Ni2O7
• Intertwined density waves in a metallic nickelate
• High-T${}_C$ superconductivity in $\mathrm{L}{\mathrm{a}}_3\mathrm{N}{\mathrm{i}}_2{\mathrm{O}}_7$ based on the bilayer two-orbital t-J model
• Intimate link between Charge Density Wave, Pseudogap and Superconducting Energy Scales in Cuprates
• Pressure Driven Fractionalization of Ionic Spins Results in Cupratelike High-$T_c$ Superconductivity in La${}_3$Ni${}_2$O${}_7$
• Superconductivity in nickelate and cuprate superconductors with strong bilayer coupling
• Pressure-enhanced spin-density-wave transition in double-layer nickelate $L{a}_{3}N{i}_2{O}_{7-\delta }$
• Competing d${}_{xy}$ and s${}_{\pm }$ Pairing Symmetries in Superconducting La${}_3$Ni${}_2$O${}_7$ emerge from LDA+FLEX Calculations
• Quenched pair breaking by interlayer correlations as a key to superconductivity in La${}_3$Ni${}_2$O${}_7$
• Pressure-enhanced splitting of density wave transitions in La${}_3$Ni${}_2$O${}_{7-\delta }$
• Effective model and $s_{\pm }$-wave superconductivity in trilayer nickelate La${}_4$Ni${}_3$O${}_{10}$
• Prediction of $s^{\pm }$-wave superconductivity enhanced by electronic doping in trilayer nickelates La${}_4$Ni${}_3$O${}_{10}$ under pressure
• Raman scattering study of Spin-Density-Wave order and electron-phonon coupling in Ba(Fe${}_{1-x}$Co${}_x$)${}_2$As${}_2$
• The electronic and magnetic structures of bilayer La${}_3$Ni${}_2$O${}_7$ at ambient pressure
• Trilayer multi-orbital models of $\mathrm{L}{\mathrm{a}}_4\mathrm{N}{\mathrm{i}}_3{\mathrm{O}}_{10}$
• Electronic structure and magnetic tendencies of trilayer La${}_4$Ni${}_3$O${}_{10}$ under pressure: structural transition, molecular orbitals, and layer differentiation
• Ultrafast Dynamics of Bilayer and Trilayer Nickelate Superconductors
• Electronic structure and magnetic correlations in trilayer nickelate superconductor La${}_4$Ni${}_3$O${}_{10}$ under pressure
• Effective model and electron correlations in trilayer nickelate superconductor La${}_4$Ni${}_3$O${}_{10}$
• Origin of the density wave instability in trilayer nickelate La${}_4$Ni${}_3$O${}_{10}$ revealed by optical and ultrafast spectroscopy
• Transition from $s_{\pm }$-wave to $d_{x^2-y^2}$-wave superconductivity driven by interlayer interaction in the bilayer two-orbital model of La${}_3$Ni${}_2$O${}_7$
• Spin-density wave and superconductivity in La${}_4$Ni${}_3$O${}_{10}$ under ambient pressure

Cited by in corpus (3)

• Electronic layer decoupling driven by density-wave order in La${}_4$Ni${}_3$O${}_{10}$
• Multiorbital character of the density wave in trilayer nickelate superconductors
• Magnetically Mediated Cross-Layer Pairing in Pressurized Trilayer Nickelate La${}_4$Ni${}_3$O${}_{10}$