High-pressure crystal growth and investigation of the metal-to-metal transition of Ruddlesden-Popper trilayer nickelates La$_4$Ni$_3$O$_{10}$

Ning Yuan; Ahmed Elghandour; Jan Arneth; Kaustav Dey; Rüdiger Klingeler

doi:10.1016/j.jcrysgro.2023.127511

paper

High-pressure crystal growth and investigation of the metal-to-metal transition of Ruddlesden-Popper trilayer nickelates La $_{4}$ Ni $_{3}$ O $_{10}$

arXiv:2311.10673 · doi:10.1016/j.jcrysgro.2023.127511

Abstract

Single crystals of Ruddlesden-Popper nickelates La $_{4}$ Ni $_{3}$ O $_{10}$ were grown by means of the floating-zone technique at oxygen pressure of 20~bar. Our results reveal the effects of the annealing process under pressure on the crystal structure. We present the requirements for crystal growth and show how a reported ferromagnetic impurity phase can be avoided. The different growth and post-annealing processes result in two distinct phases $P 2_{1} / a$ and {\it Bmab} in which the metal-to-metal transitions occur at 152~K and 136~K, respectively.

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Superconductivity in trilayer nickelate La4Ni3O10 under pressure
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Impact of Pressure and Apical Oxygen Vacancies on Superconductivity in La $_{3}$ Ni $_{2}$ O $_{7}$
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Superconductivity in La $_{4}$ Ni $_{3}$ O $_{10}$ Under Pressure
Theoretical study of the crystal structure of the bilayer nickel oxychloride Sr $_{3}$ Ni $_{2}$ O $_{5}$ Cl $_{2}$ and analysis of possible unconventional superconductivity
Origin of the Diagonal Double-Stripe Spin-Density-Wave and Potential Superconductivity in Bulk La $_{3}$ Ni $_{2}$ O $_{7}$ at Ambient Pressure
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High-pressure crystal growth and investigation of the metal-to-metal transition of Ruddlesden-Popper trilayer nickelates La4​Ni3​O10​

Abstract

References in corpus (16)

Cited by in corpus (18)

High-pressure crystal growth and investigation of the metal-to-metal transition of Ruddlesden-Popper trilayer nickelates La $_{4}$ Ni $_{3}$ O $_{10}$