Superconductivity in trilayer nickelate La4Ni3O10 under pressure

Abstract

Nickelate superconductors have attracted a great deal of attention over the past few decades due to their similar crystal and electronic structures with high-temperature cuprate superconductors. Here, we report the superconductivity in a pressurized Ruddlesden-Popper phase single crystal, La4Ni3O10 (n = 3), and its interplay with the density wave order in the phase diagram. With increasing pressure, the density wave order as indicated by the anomaly in the resistivity is progressively suppressed, followed by the emergence of the superconductivity around 25 K under I4/mmm space group. The susceptibility measurements confirm bulk superconductivity with a volume fraction exceeding 80%. Moreover, theoretical analysis unveils that antiferromagnetic (AFM) super-exchange interactions can serve as the effective pairing interaction for the emergence of superconductivity (SC) in pressurized La4Ni3O10. Our research provides a new platform for the investigation of the unconventional superconductivity mechanism in Ruddlesden-Popper trilayer perovskite nickelates.

21 pages, 4 figures

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• Role of Oxygen States in the Low Valence Nickelate La${}_4$Ni${}_3$O${}_8$

Cited by in corpus (31)

• Bulk superconductivity in pressurized trilayer nickelate Pr4Ni3O10 single crystals
• Band Structure and Pairing Nature of La${}_3$Ni${}_2$O${}_7$ Thin Film at Ambient Pressure
• Dichotomy in Low- and High-energy Band Renormalizations in Trilayer Nickelate $L{a}_{4}N{i}_3{O}_{10}$: a Comparison with Cuprates
• Out-of-plane bond-order phase, superconductivity, and their competition in the $t$-$J_{\parallel }$-$J_{\perp }$ model: Possible implications for bilayer nickelates
• Phase diagrams and two key factors to superconductivity of Ruddlesden-Popper nickelates
• Superconducting Dome in ${\mathrm{La}}_{3-x}{\mathrm{Sr}}_x{\mathrm{Ni}}_2{\mathrm{O}}_{7-\delta }$ Thin Films
• Superconductivity in La${}_4$Ni${}_3$O${}_{10}$ Under Pressure
• $t$-$J$ model for strongly correlated two-orbital systems: Application to bilayer nickelate superconductors
• Magnetic Correlations and Pairing Tendencies of the Hybrid Stacking Nickelate Superlattice La${}_7$Ni${}_5$O${}_{17}$ (La${}_3$Ni${}_2$O${}_7$/La${}_4$Ni${}_3$O${}_{10}$) under Pressure
• Origin of the Diagonal Double-Stripe Spin-Density-Wave and Potential Superconductivity in Bulk La${}_3$Ni${}_2$O${}_7$ at Ambient Pressure
• Electronic Structure, Magnetic and Pairing Tendencies of Alternating Single-layer Bilayer Stacking Nickelate La${}_5$Ni${}_3$O${}_{11}$ Under Pressure
• Complex spin-density-wave ordering in La${}_4$Ni${}_3$O${}_{10}$
• Lattice-charge coupling in a trilayer nickelate with intertwined density wave order
• Nodeless superconducting gap and electron-boson coupling in (La,Pr,Sm)${}_3$Ni${}_2$O${}_7$ films
• Variational Quantum Monte Carlo investigations of the superconducting pairing in La${}_3$Ni${}_2$O${}_7$
• General trends of electronic structures, superconducting pairing, and magnetic correlations in the Ruddlesden-Popper nickelate $m$-layered superconductors La${}_{m+1}$Ni${}_m$O${}_{3m+1}$
• Weakly anisotropic superconductivity of Pr4Ni3O10 single crystals
• Numerical study of bi-layer two-orbital model for La${}_3$Ni${}_2$O${}_7$ on a plaquette ladder
• Optical control of the crystal structure in the bilayer nickelate superconductor La3Ni2O7 via nonlinear phononics
• Decoupling between $d_{x^2-y^2}$ and $d_{z^2}$ orbitals in hole doped La${}_3$Ni${}_2$O${}_7$
• Compressive Strain Turns $s^{\pm }$ into $d$-Wave Pairing in One-unit-cell La${}_3$Ni${}_2$O${}_7$ Thin Film Via Substrate-Induced Hole Doping
• Theoretical study on the possibility of high $T_c$ s$\pm$-wave superconductivity in the heavily hole-doped infinite layer nickelates
• Electronic layer decoupling driven by density-wave order in La${}_4$Ni${}_3$O${}_{10}$
• Progress of ambient-pressure superconductivity in bilayer nickelate thin films
• Weak electronic correlations in the cobalt oxychalcogenide superconductor Na2CoSe2O
• Superconductivity in the spin-state crossover materials: Nickelates with planar-coordinated low-spin Ni${}^{2+}$ ions
• Multiorbital character of the density wave in trilayer nickelate superconductors
• Layer-Resolved Impurity States Reveal Competing Pairing Mechanisms in Trilayer Nickelate Superconductor La${}_4$Ni${}_3$O${}_{10}$
• Intertwined Charge and Spin Density Waves in Trilayer Nickelate La${}_4$Ni${}_3$O${}_{10}$ Revealed by ${}^{139}$La NQR
• $L{a}_{3}P{d}_{2}Na{O}_9$: A High-Valent Insulating Palladate
• Effect of doping on the electronic structure, orbital-dependent renormalizations, and magnetic correlations in bilayer La${}_3$Ni${}_2$O${}_7$