Dynamics of a buffer-gas-loaded, deep optical trap for molecules
arXiv:2301.12620 · doi:10.1103/PhysRevResearch.5.033008
Abstract
We describe an approach to optically trapping small, chemically stable molecules at cryogenic temperatures by buffer-gas loading a deep optical dipole trap. The ~10 K trap depth will be produced by a tightly-focused, 1064-nm cavity capable of reaching intensities of hundreds of GW/cm. Molecules will be directly buffer-gas loaded into the trap using a helium buffer gas at 1.5 K. The very far-off-resonant, quasielectrostatic trapping mechanism is insensitive to a molecule's internal state, energy level structure, and its electric and magnetic dipole moment. Here, we theoretically investigate the trapping and loading dynamics, as well as the heating and loss rates, and conclude that - molecules are likely to be trapped. Our trap would open new possibilities in molecular spectroscopy, studies of cold chemical reactions, and precision measurement, amongst other fields of physics.
arXiv comment34 pages, 7 figures
References in corpus (56)
- SciPy 1.0--Fundamental Algorithms for Scientific Computing in Python
- Search for New Physics with Atoms and Molecules
- Quantum computation with trapped polar molecules
- Quantum-State Controlled Chemical Reactions of Ultracold KRb Molecules
- Measurement of the fine-structure constant as a test of the Standard Model
- Laser cooling of a diatomic molecule
- Bose-Einstein condensation in trapped dipolar gases
- Cold molecules: Progress in Quantum Engineering of Chemistry and Quantum Matter
- Quantum State Engineering and Precision Metrology using State-Insensitive Light Traps
- The Buffer Gas Beam: An Intense, Cold, and Slow Source for Atoms and Molecules
- A Rigorous Attempt to Verify Interstellar Glycine
- Demonstration of fault-tolerant universal quantum gate operations
- A Fermi Degenerate Gas of Polar Molecules
- Sisyphus Laser Cooling of a Polyatomic Molecule
- New frontiers with quantum gases of polar molecules
- Laser Cooling of Optically Trapped Molecules
- Deceleration and electrostatic trapping of OH radicals
- Dynamical polarizability of atoms in arbitrary light fields: general theory and application to cesium
- Ultracold molecules for measuring the electron's electric dipole moment
- Magneto-Optical Trapping and Sub-Doppler Cooling of a Polyatomic Molecule
- Direct Laser Cooling of a Symmetric Top Molecule
- Strong Field Ionization Rate for Arbitrary Laser Frequencies
- Optoelectrical cooling of polar molecules to sub-millikelvin temperatures
- Robust encoding of a qubit in a molecule
- Laser-Cooled Polyatomic Molecules for Improved Electron Electric Dipole Moment Searches
- Magnetic trapping and Zeeman relaxation of imidogen (NH X-triplet-Sigma)
- Continuous probe of cold complex molecules with infrared frequency comb spectroscopy
- Photo-induced two-body loss of ultracold molecules
- 1D Magneto-Optical Trap of Polyatomic Molecules
- Sub-Doppler Cooling and Compressed Trapping of YO Molecules at K Temperatures
- Microwave traps for cold polar molecules
- Methanol as a tracer of fundamental constants
- Cold N+NH Collisions in a Magnetic Trap
- Molecular lattice clock with long vibrational coherence
- Perspective: Accurate ro-vibrational calculations on small molecules
- Collisions of ultracold molecules in bright and dark optical dipole traps
- Interatomic potentials, electric properties, and spectroscopy of the ground and excited states of the Rb_2 molecule: Ab initio calculations and effect of a non-resonant field
- Collisions between cold molecules in a superconducting magnetic trap
- A quasiclassical method for calculating the density of states of ultracold collision complexes
- A buffer gas beam source for short, intense and slow molecular pulses
- Optical cycling, radiative deflection and laser cooling of barium monohydride (BaH)
- Ultracold molecules from ultracold atoms: a case study with the KRb molecule
- High-Power Near-Concentric Fabry-Perot Cavity for Phase Contrast Electron Microscopy
- Cavity-Enhanced Rayleigh Scattering
- Evaporative cooling of a small number of atoms in a single-beam microscopic dipole trap
- A terahertz vibrational molecular clock with systematic uncertainty at the level
- Observation of the relativistic reversal of the ponderomotive potential
- Evaluation of heating effects on atoms trapped in an optical trap
- Buffer gas cooling and trapping of atoms with small magnetic moments
- Continuous 40 GW/cm laser intensity in a near-concentric optical cavity
- Absolute measurement of laser ionization yield in atmospheric pressure range gases over 14 decades
- Buffer-gas cooling of molecules in the low-density regime: Comparison between simulation and experiment
- Simulation of Cryogenic Buffer Gas Beams
- Microwave trap for atoms and molecules
- Trapping cold ground state argon atoms for sympathetic cooling of molecules
- An Electro-Optical Trap for Polar Molecules
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- Ab Initio Calculations of the Static and Dynamic Polarizability of BaOH