Observation of gigantic spin conversion anisotropy in bismuth
arXiv:2208.00589 · doi:10.1073/pnas.2215030120
Abstract
Whilst the g-factor can be anisotropic due to the spin-orbit interaction (SOI), its existence in solids cannot be simply asserted from a band structure, which hinders progress on studies from such the viewpoints. The g-factor in bismuth (Bi) is largely anisotropic; especially for holes at T-point, the g-factor perpendicular to the trigonal axis is negligibly small (< 0.112), whereas the g-factor along the trigonal axis is very large (62.7). We clarified in this work that the large g- factor anisotropy gives rise to the gigantic spin conversion anisotropy in Bi from experimental and theoretical approaches. Spin-torque ferromagnetic resonance was applied to estimate the spin conversion efficiency in rhombohedral (110) Bi to be 17%, which is unlike the negligibly small efficiency in Bi(111). Harmonic Hall measurements supports the large spin conversion efficiency in Bi(110). This is the first observation of gigantic spin conversion anisotropy as the clear manifestation of the g-factor anisotropy. Beyond the emblematic case of Bi, our study unveiled the significance of the g-factor anisotropy in condensed-matter physics and can pave a pathway toward establishing novel spin physics under g-factor control.
28 pages, 7 figures
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Cited by in corpus (5)
- Intrinsic orbital and spin Hall effect in bismuth semimetal
- Charge to spin conversion in atomically thin bismuth
- Temperature dependence of charge-to-spin conversion in rhombohedral (110) bismuth thin film
- Charge-to-spin conversion in epitaxial and polycrystalline Bi and Bi/Ag layers
- Investigating spin and orbital effects via spin-torque ferromagnetic resonance