Antiferromagnetic fluctuations and orbital-selective Mott transition in the van der Waals ferromagnet Fe3-xGeTe2

Abstract

Fe3-xGeTe2 is a layered magnetic van der Waals material of interest for both fundamental and applied research. Despite the observation of intriguing physical properties, open questions exist even on the basic features related to magnetism: is it a simple ferromagnet or are there antiferromagnetic regimes and are the moments local or itinerant. Here, we demonstrate that antiferromagnetic spin fluctuations coexist with the ferromagnetism through comprehensive elastic and inelastic neutron scattering and thermodynamic measurements. Our realistic dynamical mean-field theory calculations reveal that the competing magnetic fluctuations are driven by an orbital selective Mott transition, where only the plane-perpendicular a1g orbital of the Fe(3d) manifold remains itinerant. Our results highlight the multi-orbital character in Fe3-xGeTe2 that supports a rare coexistence of local and itinerant physics within this material.

arXiv comment16 pages, 3 main figures

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• Manifestation of incoherent-coherent crossover and non-Stoner magnetism in the electronic structure of Fe${}_3$GeTe${}_2$
• Direct evidence from high-field magnetotransport for a dramatic change of quasiparticle character in van der Waals ferromagnet Fe${}_{3-x}$GeTe${}_2$
• Magnetic excitations and absence of charge order in the van der Waals ferromagnet Fe${}_{4.75}$GeTe${}_2$
• Magnon Damping as a Probe of Kondo Coupling in Magnetically Ordered Systems
• Signatures of Kondo-lattice behavior in the two-dimensional ferromagnet Fe${}_3$GeTe${}_2$