Direct evidence from high-field magnetotransport for a dramatic change of quasiparticle character in van der Waals ferromagnet Fe${}_{3-x}$GeTe${}_2$

Abstract

Magnetometry and magnetoresistance (MR) data taken on the van der Waals ferromagnet Fe${}_{3-x}$GeTe${}_2$ (FGT) reveal three distinct contributions to the MR: a linear negative component, a contribution from closed Fermi-surface orbits, and a $H^2$ enhancement linked to a non-coplanar spin arrangement. Contrary to earlier studies on FGT, by accounting for the field dependence of the anomalous Hall effect, we find that the ordinary Hall coefficient decreases markedly below 80 K, indicating a significant change in character of the electrons and holes on the Fermi surface at this temperature. The resulting altered ground state eventually causes the Hall coefficient to reverse sign at 35 K. Our Hall data support the proposal that Kondo-lattice behavior develops in this $d$-electron material below 80 K. Additional evidence comes from the negative linear component of the MR, which arises from electron-magnon scattering with an atypical temperature dependence attributable to the onset of Kondo screening.

References in corpus (10)

• Van der Waals heterostructures for spintronics and opto-spintronics
• Van der Waals heterostructures for high-performance device applications: challenges and opportunities
• Antisymmetric magnetoresistance in van der Waals Fe3GeTe2/graphite/Fe3GeTe2 tri-layer heterostructures
• Large anomalous Nernst effect in a van der Waals ferromagnet Fe${}_3$GeTe${}_2$
• Neutron spectroscopy evidence on the dual nature of magnetic excitations in a van der Waals metallic ferromagnet Fe${}_{2.72}$GeTe${}_2$
• Effects of Fe deficiency and Co substitution in polycrystalline and single crystals of Fe${}_3$GeTe${}_2$
• Antiferromagnetic fluctuations and orbital-selective Mott transition in the van der Waals ferromagnet Fe3-xGeTe2
• Relating spin-polarized STM imaging and inelastic neutron scattering in the van-der-Waals ferromagnet Fe3GeTe2
• Observation of flat bands due to band hybridization in 3d-electron heavy-fermion compound CaCu3Ru4O12
• An emerging global picture of heavy fermion physics