Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure
arXiv:2105.01312
Abstract
Quantum confinement in atomically-thin TMDCs enables the realization of deterministic single-photon emitters. The position and polarization control of single photons have been achieved via local strain engineering using nanostructures. However, most existing TMDC-based emitters are operated by optical pumping, while the emission sites in electrically pumped emitters are uncontrolled. Here, we demonstrate electrically driven single-photon emitters located at the positions where strains are induced by atomic-force-microscope indentation on a van der Waals heterostructure consisting of graphene, hexagonal-boron nitride, and tungsten diselenide. The optical, electrical, and mechanical properties induced by the local strain gradient were systematically analyzed. In particular, single-photon emission was observed at the indentation sites at 4 K. The emission exhibits photon anti-bunching behavior with a g(2)(0) value of ~0.3, intensity saturation and a linearly cross-polarized doublet. This robust spatial control of electrically driven single-photon emitters will pave the way for the practical implementation of integrated quantum light sources.
arXiv comment29 pages, 8 figures
References in corpus (11)
- Van der Waals heterostructures
- Light-emitting diodes by bandstructure engineering in van der Waals heterostructures
- Optoelectronics with electrically tunable PN diodes in a monolayer dichalcogenide
- Solar-energy conversion and light emission in an atomic monolayer p-n diode
- Large-scale quantum-emitter arrays in atomically thin semiconductors
- Deterministic strain-induced arrays of quantum emitters in a two-dimensional semiconductor
- Atomically thin quantum light emitting diodes
- Integration of Single Photon Emitters in 2D Layered Materials with a Silicon Nitride Photonic Chip
- Localized inter-valley defect excitons as single-photon emitters in WSe
- Coupling single photons from discrete quantum emitters in WSe to lithographically defined plasmonic slot-waveguides
- Coupling emission from single localized defects in 2D semiconductor to surface plasmon polaritons