Collective excitations in twisted bilayer graphene close to the magic angle
arXiv:1910.07893 · doi:10.1038/s41567-021-01327-8
Abstract
The electronic properties of twisted bilayer graphene (TBG) can be dramatically different from those of a single graphene layer, in particular when the two layers are rotated relative to each other by a small angle. TBG has recently attracted a great deal of interest, sparked by the discovery of correlated insulating and superconducting states, for twist angle close to a so-called 'magic angle' . In this work, we unveil, via near-field optical microscopy, a collective plasmon mode in charge-neutral TBG near the magic angle, which is dramatically different from the ordinary single-layer graphene intraband plasmon. In selected regions of our samples, we find a gapped collective mode with linear dispersion, akin to the bulk magnetoplasmons of a two-dimensional (2D) electron gas. We interpret these as interband plasmons and associate those with the optical transitions between quasi-localized states originating from the moiré superlattice. Surprisingly, we find a higher plasmon group velocity than expected, which implies an enhanced strength of the corresponding optical transition. This points to a weaker interlayer coupling in the AA regions. These intriguing optical properties offer new insights, complementary to other techniques, on the carrier dynamics in this novel quantum electron system.
arXiv comment36 pages, 15 figures
References in corpus (56)
- Magic-angle graphene superlattices: a new platform for unconventional superconductivity
- Boron nitride substrates for high-quality graphene electronics
- Correlated Insulator Behaviour at Half-Filling in Magic Angle Graphene Superlattices
- Moire bands in twisted double-layer graphene
- Graphene plasmonics: A platform for strong light-matter interaction
- Tuning superconductivity in twisted bilayer graphene
- Energy gaps, topological insulator state and zero-field quantum Hall effect in graphene by strain engineering
- Emergent ferromagnetism near three-quarters filling in twisted bilayer graphene
- Superconductors, Orbital Magnets, and Correlated States in Magic Angle Bilayer Graphene
- Graphene bilayer with a twist: electronic structure
- Intrinsic quantized anomalous Hall effect in a moiré heterostructure
- Polaritons in layered 2D materials
- Observation of Van Hove singularities in twisted graphene layers
- Highly confined low-loss plasmons in graphene-boron nitride heterostructures
- Sub-diffractional, volume-confined polaritons in a natural hyperbolic material: hexagonal boron nitride
- Magic Angle Spectroscopy
- Flat Bands in Slightly Twisted Bilayer Graphene
- Origin of Magic Angles in Twisted Bilayer Graphene
- Atomic and electronic reconstruction at van der Waals interface in twisted bilayer graphene
- Imaging Electronic Correlations in Twisted Bilayer Graphene near the Magic Angle
- Electric Field Tunable Correlated States and Magnetic Phase Transitions in Twisted Bilayer-Bilayer Graphene
- Charge-Order and Broken Rotational Symmetry in Magic Angle Twisted Bilayer Graphene
- Spectroscopic signatures of many-body correlations in magic angle twisted bilayer graphene
- Continuum Model of the Twisted Bilayer
- Spin-polarized Correlated Insulator and Superconductor in Twisted Double Bilayer Graphene
- Twistable electronics with dynamically rotatable heterostructures
- Lattice relaxation and energy band modulation in twisted bilayer graphenes
- Evidence of Gate-Tunable Mott Insulator in Trilayer Graphene-Boron Nitride Moiré Superlattice
- Correlated states in twisted double bilayer graphene
- Optical Absorption in Twisted Bilayer Graphene
- Superlattice-induced insulating states and valley-protected orbits in twisted bilayer graphene
- Mapping the twist angle and unconventional Landau levels in magic angle graphene
- Photonic crystals for nano-light in moiré graphene superlattices
- Light-matter interactions with photonic quasiparticles
- Energy Spectrum and Quantum Hall Effect in Twisted Bilayer Graphene
- Ultra-confined acoustic THz graphene plasmons revealed by photocurrent nanoscopy
- Electrostatic effects, band distortions and superconductivity in twisted graphene bilayers
- An exact continuum model for low-energy electronic states of twisted bilayer graphene
- Non-Abelian gauge potentials in graphene bilayers
- Mechanical cleaning of graphene
- Ultraviolet and visible range plasmonics of a topological insulator
- Electronic Compressibility of Magic-Angle Graphene Superlattices
- Infrared Reflectance Spectrum of BN Calculated from First Principles
- Relative efficiency of polariton emission in two-dimensional materials
- Optical conductivity, Drude weight and plasmons in twisted graphene bilayers
- Intrinsic plasmons in 2D Dirac materials
- Optical Conductivity of Twisted Bilayer Graphene
- Quasi-flat plasmonic bands in twisted bilayer graphene
- Strong plasmon reflection at nanometer-size gaps in monolayer graphene on SiC
- Intrinsically Undamped Plasmon Modes in Narrow Electron Bands
- Plasmon reflections by topological electronic boundaries in bilayer graphene
- Real-space imaging of the tailored plasmons in twisted bilayer graphene
- Optical and plasmonic properties of twisted bilayer graphene: Impact of interlayer tunneling asymmetry and ground-state charge inhomogeneity
- Superconductivity from collective excitations in magic angle twisted bilayer graphene
- Correlated states in magic angle twisted bilayer graphene under the optical conductivity scrutiny
- A Twisted Pair Cryogenic Filter
Cited by in corpus (46)
- Twisted Nano-optics: Manipulating Light at the Nanoscale with Twisted Phonon Polaritonic Slabs
- Quantum Nanophotonics in Two-Dimensional Materials
- Multiple and spectrally robust photonic magic angles in reconfigurable α-MoO3 trilayers
- Hydrodynamic approach to two-dimensional electron systems
- Roadmap for Photonics with 2D Materials
- Chiral plasmons with twisted atomic bilayers
- Kondo Lattice Model of Magic-Angle Twisted-Bilayer Graphene: Hund's Rule, Local-Moment Fluctuations, and Low-Energy Effective Theory
- A perspective of twisted photonic structures
- Tunable moiré materials for probing Berry physics and topology
- Symmetric Kondo Lattice States in Doped Strained Twisted Bilayer Graphene
- Dynamical correlations and order in magic-angle twisted bilayer graphene
- Terahertz photogalvanics in twisted bilayer graphene close to the second magic angle
- Roadmap on Nonlocality in Photonic Materials and Metamaterials
- Unconventional Nonlocal Relaxation Dynamics in a Twisted Graphene Moire Superlattice
- Cryogenic Magneto-Terahertz Scanning Near-field Optical Microscope (cm-SNOM)
- TBG as Topological Heavy Fermion: II. Analytical approximations of the model parameters
- Plasmon-enhanced near-field chirality in twisted van der Waals heterostructures
- Flat-band plasmons in twisted bilayer transition metal dichalcogenides
- Quantum plasmonic non-reciprocity in parity-violating magnets
- Tunable interband and intraband plasmons in twisted double bilayer graphene
- Polaritonic Quantum Matter
- Non-coplanar magnetism, topological density wave order and emergent symmetry at half-integer filling of moiré Chern bands
- Theory of intrinsic acoustic plasmons in twisted bilayer graphene
- Intrinsic nonreciprocal bulk plasmons in noncentrosymmetric magnetic systems
- Moiré-Induced Transport in CVD-Based Small-Angle Twisted Bilayer Graphene
- Infrared photoresistance as a sensitive probe of electronic transport in twisted bilayer graphene
- Tuning flat bands by interlayer interaction, spin-orbital coupling, and external fields in twisted homotrilayer MoS
- Neutral magic-angle bilayer graphene: Condon instability and chiral resonances
- Stacking-induced magnetic frustration and spiral spin liquid
- Many-body perturbation theory for moiré systems
- Moiré fractals in twisted graphene layers
- Magnetoplasmons in magic-angle twisted bilayer graphene
- Cascades in transport and optical conductivity of Twisted Bilayer Graphene
- Interlayer Hopping between Surface Mott Insulator and Bulk Band Insulator in layered 1T-TaS_{2}
- Emergent Hyper-Magic Manifold in Twisted Kitaev Bilayers
- Towards tunable graphene phononic crystals
- Ferromagnetism vs. Antiferromagnetism in Narrow-Band Systems: Competition Between Quantum Geometry and Band Dispersion
- Quantum geometry induced microwave enhancement of flat band superconductivity
- Collective excitations of the Chern-insulator states in commensurate double moiré superlattices of twisted bilayer graphene on hexagonal boron nitride
- Mean-field Modelling of Moiré Materials: A User's Guide with Selected Applications to Twisted Bilayer Graphene
- Strongly Coupled Exciton--Hyperbolic-phonon-polariton Hybridized States in hBN-encapsulated Biased Bilayer Graphene
- Large quantum nonreciprocity in plasmons dragged by drifting electrons
- Interaction-mitigated Landau damping
- Magic angle and plasmon mode engineering in twisted trilayer graphene with pressure
- Terahertz magneto-nanoscopy of encapsulated monolayer graphene
- Interband plasmons due to Mexican hat dispersion in two-dimensional materials with inverted bands