Symmetric Kondo Lattice States in Doped Strained Twisted Bilayer Graphene

H. Hu; G. Rai; L. Crippa; J. Herzog-Arbeitman; D. Călugăru; T. Wehling; G. Sangiovanni; R. Valenti; A. M. Tsvelik; B. A. Bernevig

doi:10.1103/PhysRevLett.131.166501

paper

Symmetric Kondo Lattice States in Doped Strained Twisted Bilayer Graphene

arXiv:2301.04673 · doi:10.1103/PhysRevLett.131.166501

Abstract

We use the topological heavy fermion (THF) model and its Kondo Lattice (KL) formulation to study the symmetric Kondo state in twisted bilayer graphene. Via a large-N approximation, we find a symmetric Kondo (SK) state in KL mode at fillings $ν = 0, \pm 1, \pm 2$ . In the SK state, all symmetries are preserved and the local moments are Kondo screened by the conduction electrons. At the mean-field level of the THF model at $ν = 0, \pm 1, \pm 2, \pm 3$ , we also find a similar symmetric state. We study the stability of the symmetric state by comparing its energy with the ordered states and find the ordered states to have lower energy. However, moving away from integer fillings by doping holes to the light bands, we find the energy difference is reduced, which suggests the loss of ordering and a tendency towards Kondo screening. In order to include many-body effects beyond the mean-field approximation, we perform dynamical mean-field theory (DMFT) calculations on the THF model. We find the spin susceptibility follows a Curie behavior at $ν = 0, \pm 1, \pm 2$ down to $\sim 2 K$ where the onset of screening of the local moment becomes visible. This hints to very low Kondo temperatures at these fillings, in agreement with the outcome of our mean-field calculations. At non-integer filling $ν = \pm 0.5, \pm 0.8, \pm 1.2$ DMFT shows deviations from a $1/ T$ -susceptibility at much higher temperatures, suggesting a more effective screening of local moments with doping. Finally, we study the effect of a $C_{3 z}$ -rotational-symmetry-breaking strain via mean-field approaches and find that a symmetric phase (that only breaks $C_{3 z}$ symmetry) can be stabilized at sufficiently large strain at $ν = 0, \pm 1, \pm 2$ . Our results suggest that a symmetric Kondo phase is strongly suppressed at integer fillings, but could be stabilized either at non-integer fillings or by applying strain.

40 pages, 15 figures

Symmetric Kondo Lattice States in Doped Strained Twisted Bilayer Graphene

Abstract

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