Nonlinear Optical Conductivity in Graphene and other 2-Band 2-D Materials

Abstract

Graphene, Silicene, ${\mathrm{MoS}}_2$ and other similar two-dimensional structures have unusual electronic properties that lend themselves to exotic device applications. These properties emanate from the fact that the electrons are endowed with Dirac fermion-like attributes. Thus these materials are not only characterized by certain fundamental principles, they also have amazing practical uses. Our emphasis here is on one such basic property concerning nonlinear response to time-dependent electric fields. We set up a first principle quantum master equation for the underlying density operator which is based on microscopic interactions between the Dirac electron with phonons and other electrons. While such an equation has general applicability to a variety of non-equilibrium phenomena in two-band systems, we focus onto the case of nonlinear optical conductivity. The derived results are separately analyzed for graphene, silicene and ${\mathrm{MoS}}_2$, and comparison made with other known results.

10 pages, 3 figures

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