Variational approach for impurity dynamics at finite temperature

Abstract

We present a general variational principle for the dynamics of impurity particles immersed in a quantum-mechanical medium. By working within the Heisenberg picture and constructing approximate time-dependent impurity operators, we can take the medium to be in any mixed state, such as a thermal state. Our variational method is consistent with all conservation laws and, in certain cases, it is equivalent to a finite-temperature Green's function approach. As a demonstration of our method, we consider the dynamics of heavy impurities that have suddenly been introduced into a Fermi gas at finite temperature. Using approximate time-dependent impurity operators involving only one particle-hole excitation of the Fermi sea, we find that we can successfully model the results of recent Ramsey interference experiments on ${}^{40}$K atoms in a ${}^6$Li Fermi gas [M.~Cetina et al., Science \textbf{354}, 96 (2016)]. We also show that our approximation agrees well with the exact solution for the Ramsey response of a fixed impurity at finite temperature. Our approach paves the way for the investigation of impurities with dynamical degrees of freedom in arbitrary quantum-mechanical mediums.

4 pages of main text with a 5-page supplementary material (SM); 2 figures in the main text and another 3 in the SM