Quasiparticle Breakdown and Spin Hamiltonian of the Frustrated Quantum Pyrochlore Yb${}_2$Ti${}_2$O${}_7$ in Magnetic Field

Abstract

The frustrated pyrochlore magnet Yb${}_2$Ti${}_2$O${}_7$ has the remarkable property that it orders magnetically, but has no propagating magnons over wide regions of the Brillouin zone. Here we use inelastic neutron scattering to follow how the spectrum evolves in cubic-axis magnetic fields. At high fields we observe in addition to dispersive magnons also a two-magnon continuum, which grows in intensity upon reducing the field and overlaps with the one-magnon states at intermediate fields leading to strong renormalization of the dispersion relations, and magnon decays. Using heat capacity measurements we find that the low and high field regions are smoothly connected with no sharp phase transition, with the spin gap increasing monotonically in field. Through fits to an extensive data set we re-evaluate the spin Hamiltonian finding dominant quantum exchange terms, which we propose are responsible for the anomalously strong fluctuations and quasiparticle breakdown effects observed at low fields.

5 pages main text + 19 pages supplemental material

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• Quasiparticle Breakdown and Spin Hamiltonian of the Frustrated Quantum Pyrochlore Yb${}_2$Ti${}_2$O${}_7$ in Magnetic Field
• Impact of Stoichiometry of Yb2Ti2O7 on its Physical Properties
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