paper

Trajectory analysis of high-harmonic generation from periodic crystals

arXiv:1611.08033 · doi:10.1103/PhysRevA.95.043416

Abstract

We theoretically study high-harmonic generation (HHG) from solids driven by intense laser pulses using a one-dimensional model periodic crystal. By numerically solving the time-dependent Schrödinger equation directly on a real-space grid, we successfully reproduce experimentally observed unique features of solid-state HHG such as the linear cutoff-energy scaling and the sudden transition from a single- to multiple-plateau structure. Based on the simulation results, we propose a simple model that incorporates vector-potential-induced intraband displacement, interband tunneling, and recombination with the valence-band hole. One key parameter is the valley-to-peak amplitude of the pulse vector potential, which determines the crystal momentum displacement during the half cycle. When the maximum peak-to-valley amplitude reaches the half width of the Brillouin zone with being the lattice constant, the HHG spectrum exhibits a transition from a single- to multiple-plateau structure, and even further plateaus appear at . The multiple cutoff positions are given as functions of and the second maximum , in terms of the energy difference between different bands. Using our recipe, one can draw electron trajectories in the momentum space, from which one can deduce, for example, the time-frequency structure of HHG without elaborate quantum-mechanical calculations. Finally, we reveal that the cutoff positions depend on not only the intensity and wavelength of the pulse, but also its duration, in marked contrast to the gas-phase case. Our model can be viewed as a solid-state and momentum-space counterpart of the familiar three-step model, highly successful for gas-phase HHG, and provide a unified basis to understand HHG from solid-state materials and gaseous media.

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