Analytical WKB theory for high-harmonic generation and its application to massive Dirac electrons

Abstract

We propose an analytical approach to high-harmonic generation (HHG) for nonperturbative low-frequency and high-intensity fields based on the (Jeffreys-)Wentzel-Kramers-Brillouin (WKB) approximation. By properly taking into account Stokes phenomena of WKB solutions, we obtain wavefunctions that systematically include the repetitive dynamics of production and acceleration of electron-hole pairs and quantum interference due to phase accumulation between different pair production times (Stückelberg phase). Using the obtained wavefunctions without relying on any phenomenological assumptions, we explicitly compute electric current (including intra- and inter-band contributions) as the source of HHG for a massive Dirac system in (1+1)-dimensions under an ac electric field. We demonstrate that the WKB approximation agrees well with numerical results obtained by solving the time-dependent Schrödinger equation and point out that the quantum interference is important in HHG. We also predict in the deep nonperturbative regime that (1) harmonic intensities oscillate with respect to electric-field amplitude $E_0$ and frequency $\Omega$, with a period determined by the Stückelberg phase; (2) the cutoff order of HHG is determined by $2e{E}_0/\hslash {\Omega }^2$, with $e$ being the electron charge; and that (3) non-integer harmonics, controlled by the Stückelberg phase, appear as a transient effect. Our WKB theory is particularly suited for a parameter regime, where the Keldysh parameter $\gamma =(\Delta /2)\Omega /e{E}_0$, with $\Delta$ being the gap size, is small. This parameter regime corresponds to intense lasers in the terahertz regime for realistic massive Dirac materials. Our analysis implies that the so-called HHG plateau can be observed at the terahertz frequency within the current technology.

5+5 pages, 3 figures; v2: discussion on cutoff law improved, experimental realization with terahertz lasers discussed, to be published in PRB Letter

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