The magnetic precursor of the pressure-induced superconductivity in Fe-ladder compound

Abstract

The pressure effects on the antiferromagentic orders in iron-based ladder compounds CsFe${}_2$Se${}_3$ and BaFe${}_2$S${}_3$ have been studied using neutron diffraction. With identical crystal structure and similar magnetic structures, the two compounds exhibit highly contrasting magnetic behaviors under moderate external pressures. In CsFe${}_2$Se${}_3$ the ladders are brought much closer to each other by pressure, but the stripe-type magnetic order shows no observable change. In contrast, the stripe order in BaFe${}_2$S${}_3$, undergoes a quantum phase transition where an abrupt increase of N$\acute{e}$el temperature by more than 50$\%$ occurs at about 1 GPa, accompanied by a jump in the ordered moment. With its spin structure unchanged, BaFe${}_2$S${}_3$ enters an enhanced magnetic phase that bears the characteristics of an orbital selective Mott phase, which is the true neighbor of superconductivity emerging at higher pressures.

arXiv comment5 pages, 4 figures, 1 table Accepted for publication on Physical Review Letters

References in corpus (21)

• Kinetic frustration and the nature of the magnetic and paramagnetic states in iron pnictides and iron chalcogenides
• Antiferromagnetic order and spin dynamics in iron-based superconductors
• Magnetism and its microscopic origin in iron-based high-temperature superconductors
• High Temperature Superconductivity in Iron Pnictides and Chalcogenides
• A Novel Large Moment Antiferromagnetic Order in K0.8Fe1.6Se2 Superconductor
• Janus-faced influence of the Hund's rule coupling in strongly correlated materials
• Spin freezing transition and non-Fermi-liquid self-energy in a 3-orbital model
• Orbital-Selective Mott transition out of band degeneracy lifting
• Pressure-induced Superconductivity in the Iron-based Ladder Material BaFe2S3
• High-spin to low-spin and orbital polarization transitions in multiorbital Mott systems
• Hund's coupling key role in multi-orbital correlations
• Orbital Selective Magnetism in the Spin-Ladder Iron Selenides Ba${}_{1-x}$K${}_x$Fe${}_2$Se${}_3$
• Block magnetism coupled with local distortion in the iron-based spin-ladder compound BaFe2Se3
• Block magnetic excitations in the orbitally selective Mott insulator BaFe2Se3
• Origin of the high Neel temperature in SrTcO3
• Exotic magnetic order in the orbital-selective Mott regime of multiorbital systems
• Magnetic States of the Two-Leg Ladder Alkali Metal Iron Selenides $A$Fe${}_2$Se${}_3$
• Ab initio downfolding study of the iron-based ladder superconductor BaFe${}_2$S${}_3$
• First-principles study of magnetic properties in Fe-ladder compound BaFe2S3
• Crystal Structure of BaFe2Se3 as a Function of Temperature and Pressure: Phase Transition Phenomena and High-Order Expansion of Landau Potential
• Coexistence of localized and itinerant electrons in BaFe2X3 (X = S and Se) revealed by photoemission spectroscopy

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