Gradual Enhancement of Stripe-Type Antiferromagnetism in Spin Ladder Material BaFe${}_2$S${}_3$ Under Pressure

Abstract

We report pressure-dependent neutron diffraction and muon spin relaxation/rotation measurements combined with first-principles calculations to investigate the structural, magnetic, and electronic properties of BaFe${}_2$S${}_3$ under pressure. The experimental results reveal a gradual enhancement of the stripe-type ordering temperature with increasing pressure up to 2.6 GPa and no observable change in the size of the ordered moment. The ab initio calculations suggest that the magnetism is highly sensitive to the Fe-S bond lengths and angles, clarifying discrepancies with previously published results. In contrast to our experimental observations, the calculations predict a monotonic reduction of the ordered moment with pressure. We suggest that the robustness of the stripe-type antiferromagnetism is due to strong electron correlations not fully considered in the calculations.

References in corpus (27)

• The Puzzle of High Temperature Superconductivity in Layered Iron Pnictides and Chalcogenides
• High-temperature superconductivity in iron-based materials
• Antiferromagnetic order and spin dynamics in iron-based superconductors
• musrfit: A free platform-independent framework for muSR data analysis
• High Temperature Superconductivity in Iron Pnictides and Chalcogenides
• Iron-Based Superconductors: current status of materials and pairing mechanism
• The Unexpected Properties of Alkali Metal Iron Selenide Superconductors
• Pressure-induced Superconductivity in the Iron-based Ladder Material BaFe2S3
• Low-energy microscopic models for iron-based superconductors: a review
• Iron Displacements and Magnetoelastic Coupling in the Spin-Ladder Compound BaFe2Se3
• Orbital Selective Magnetism in the Spin-Ladder Iron Selenides Ba${}_{1-x}$K${}_x$Fe${}_2$Se${}_3$
• BaFe${}_2$Se${}_3$: a high $T_{\mathrm{C}}$ magnetic multiferroic with large ferrielectric polarization
• Block magnetic excitations in the orbitally selective Mott insulator BaFe2Se3
• Emergent loop-nodal s${}_{\pm }$-wave superconductivity in CeCu${}_2$Si${}_2$: similarities to the iron-based superconductors
• Sequential structural and antiferromagnetic transitions in BaFe${}_2$Se${}_3$ under pressure
• Pressure-driven phase transition from antiferromagnetic semiconductor to nonmagnetic metal in two-leg ladders $A$Fe${}_2$$X$${}_3$ ($A$=Ba or K, $X$=S or Se)
• The magnetic precursor of the pressure-induced superconductivity in Fe-ladder compound
• Synthesis, crystal and magnetic structure of iron selenide BaFe2Se3 with possible superconductivity at Tc=11K
• Magnetic properties and pairing tendencies of the iron-based superconducting ladder BaFe${}_2$S${}_3$: combined ab initio and density matrix renormalization group study
• Orbital order and fluctuations in the two-leg ladder materials BaFe${}_2{X}_3$ ($X$ = S and Se) and CsFe${}_2$Se${}_3$
• Ab initio downfolding study of the iron-based ladder superconductor BaFe${}_2$S${}_3$
• First-principles study of magnetic properties in Fe-ladder compound BaFe2S3
• Pairing Tendencies in a Two-orbital Hubbard Model in One Dimension
• Coexistence of localized and itinerant electrons in BaFe2X3 (X = S and Se) revealed by photoemission spectroscopy
• Strong ferromagnetic exchange interaction in the parent state of the superconductivity in BaFe${}_2$S${}_3$
• Two spatially separated phases in semiconducting Rb${}_{0.8}$Fe${}_{1.5}$S${}_2$
• Phase competition in a one-dimensional three-orbital Hubbard-Holstein model

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• Robust block magnetism in the spin ladder compound BaFe${}_2$Se${}_3$ under hydrostatic pressure
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• Non-superconducting electronic ground state in pressurized BaFe${}_2$S${}_3$ and BaFe${}_2$S${}_{2.5}$Se${}_{0.5}$
• Structural, magnetic, and electronic evolution of the spin-ladder system BaFe${}_2$S${}_{3-x}$Se${}_x$ with isoelectronic substitution
• Dichotomy Between Orbital and Magnetic Nematic Instabilities in BaFe2S3
• An \textit{ab initio} study of magnetic structure transitions of FePS${}_3$ under high pressure
• The role of the nominal iron content in the structural, compositional and physical properties of BaFe${}_{2+\delta }$S${}_3$
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