Ferro-orbital ordering transition in iron telluride Fe${}_{1+y}$Te

Abstract

Fe${}_{1+y}$Te with $y\lesssim 0.05$ exhibits a first-order phase transition on cooling to a state with a lowered structural symmetry, bicollinear antiferromagnetic order, and metallic conductivity, $d\rho /dT>0$. Here, we study samples with $y=0.09(1)$, where the frustration effects of the interstitial Fe decouple different orders, leading to a sequence of transitions. While the lattice distortion is closely followed by \emph{incommensurate} magnetic order, the development of \emph{bicollinear} order and metallic electronic coherence is uniquely associated with a separate hysteretic first-order transition, at a markedly lower temperature, to a phase with dramatically enhanced bond-order wave (BOW) order. The BOW state suggests ferro-orbital ordering, where electronic delocalization in ferromagnetic zigzag chains decreases local spin and results in metallic transport.

arXiv comment5 pages, 4 figures

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