Atomic Rydberg Reservoirs for Polar Molecules

Abstract

We discuss laser dressed dipolar and Van der Waals interactions between atoms and polar molecules, so that a cold atomic gas with laser admixed Rydberg levels acts as a designed reservoir for both elastic and inelastic collisional processes. The elastic scattering channel is characterized by large elastic scattering cross sections and repulsive shields to protect from close encounter collisions. In addition, we discuss a dissipative (inelastic) collision where a spontaneously emitted photon carries away (kinetic) energy of the collision partners, thus providing a significant energy loss in a single collision. This leads to the scenario of rapid thermalization and cooling of a molecule in the mK down to the μK regime by cold atoms.

6 pages, 4 figures

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Cited by in corpus (25)

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• Manipulation of Molecules with Electromagnetic Fields
• Variational principle for steady states of dissipative quantum many-body systems
• Thermodynamics of quantum systems under dynamical control
• Driven-dissipative dynamics of a strongly interacting Rydberg gas
• Dissipative Binding of Lattice Bosons through Distance-Selective Pair Loss
• A Rydberg-dressed Magneto-Optical Trap
• Observation of Rydberg blockade due to the charge-dipole interaction between an atom and a polar molecule
• Electrically tuned Förster resonances in collisions of NH${}_3$ with Rydberg He atoms
• Atomic self-organization emerging from tunable quadrature coupling
• Rydberg-State-Resolved Resonant Energy Transfer in Cold Electric-Field-Controlled Intrabeam Collisions of NH${}_3$ with Rydberg He Atoms
• Controlling ultracold chemical reactions via Rydberg-dressed interactions
• Two-body interactions and decay of three-level Rydberg-dressed atoms
• Quantum transport in chemically functionalized graphene at high magnetic field: Defect-Induced Critical States and Breakdown of Electron-Hole Symmetry
• State resolved investigation of Förster resonant energy transfer in collisions between polar molecules and Rydberg atoms
• Optical control of atom-ion collisions using a Rydberg state
• Probing resonant energy transfer in collisions of ammonia with Rydberg helium atoms by microwave spectroscopy
• Quantum melting of two-component Rydberg crystals
• Rydberg atom-enabled spectroscopy of polar molecules via Förster resonance energy transfer
• Sympathetic cooling and slowing of molecules with Rydberg atoms
• Preparation of Knill-Lafamme-Milburn states based on superconducting qutrits
• $C_6$ coefficients for interacting Rydberg atoms and alkali-metal dimers
• Quantum Zeno-based Detection and State Engineering of Ultracold Polar Molecules
• Probing van der Waals interactions and detecting polar molecules by Förster resonance energy transfer with Rydberg atoms at temperatures below 100 mK
• Quantum criticality and factorization in a constrained Rydberg spin chain