Specific heat and upper critical field in KFe2As2 single crystals

Abstract

We report low-temperature specific heat measurements for high-quality single crystalline KFe2As2 (T_c about 3.5 K). The investigated zero-field specific heat data yields an unusually large nominal Sommerfeld coefficient gamma_n of 94(3) mJ/mol K^2 which is however significantly affected by extrinsic contributions as evidenced by a sizable residual linear specific heat and various theoretical considerations including also an analysis of Kadowaki-Woods relations. Then KFe2As2 should be classified as a weak to intermediately strong coupling superconductor with a total electron-boson coupling constant lambda_tot near 1 (including a calculated weak electron-phonon coupling constant of lambda_el-ph =0.17. From specific heat and ac susceptibility studies in external magnetic fields the magnetic phase diagram has been constructed. We confirm the high anisotropy of the upper critical fields B_c2(T) ranging from a factor of 5 near T_c to a slightly reduced value approaching T=0 for fields B || ab$ and || c and show that their ratio Gamma slightly exceeds the mass anisotropy of 4.35 derived from our full-relativistic LDA-band structure calculations. Its slight reduction when approaching T=0 is not a consequence of Pauli-limiting as in less perfect samples but point likely to a multiband effect. We also report irreversibility field data obtained from ac susceptibility measurements. The double-maximum in the T-dependence of its imaginary part for fields B || c indicates a peak-effect in the T-dependence of critical currents.

12 pages, 8 fiqures (2 new figures) specific heat raw-data corrected, estimates for a reduced electronic specific heat added, extended theoretical analysis, 2 new authors included

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