paper

Crossover in the magnetic response of single-crystalline BaKFeAs and Lifshitz critical point evidenced by Hall effect measurements

arXiv:1411.7906 · doi:10.1103/PhysRevB.90.224508

Abstract

We report the doping evolution of magnetic susceptibility and Hall coefficient in high quality BaKFeAs () single crystals. It is found that the normal-state magnetic susceptibility of BaKFeAs compounds undergoes a crossover from linear- dependence in the undoped and underdoped samples into KFeAs-type magnetic response in the overdoped samples with increasing K content. Hall coefficient of underdoped sample =0.22 shows a rapid increase above spin-density-wave transition temperature . Below , it increases slowly. of optimally doped and slightly overdoped samples () shows relative weak temperature dependence and saturation tendency below 150 K. However, of K heavily overdoped samples () increases rapidly below 150 K. Meanwhile, Hall angle displays a concave temperature dependence within the doping range , whereas it changes to a convex temperature dependence within the doping range . The dramatic change coincides with Lifshitz transition occurred around the critical doping =0.80, where ARPES measurements had confirmed that electron pocket disappears with excess hole doping in BaKFeAs system. It is suggested that the characteristic temperature * at around K observed in susceptibility and Hall coefficient, as well as previously reported resistivity data, may indicate an incoherence-coherence crossover in BaKFeAs system.

to be published in Phys. Rev. B

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