Mass renormalization in the band width-controlled Mott-Hubbard systems SrVO3 and CaVO3 studied by angle-resolved photoemission spectroscopy

Abstract

Ca1-xSrxVO3 is a Mott-Hubbard-type correlated electron system whose bandwidth can be varied by the V-O-V bond angle, but the actual effect of bandwidth control on the electronic structure has been controversial in previous photoemission experiments. In this work, band dispersions and Fermi surfaces of SrVO3 and CaVO3 are studied by angle-resolved photoemission spectroscopy. Near the Fermi level (EF), three bands forming cylindricalFermi surfaces derived from the three V 3d t2g orbitals have been observed. The observed band widths for both compounds are almost half of those predicted by local-density-approximation band-structure calculation, confirming mass renormalization caused by electron correlation. It has been clearly demonstrated that the width of the d band in CaVO3 is narrower than that in SrVO3, qualitatively consistent with the result of band-structure calculation. Roles of the orthorhombic lattice distortion and electron correlation in the observed band narrowing are discussed.

13 pages, 5 figures

References in corpus (7)

• Mott transition and suppression of orbital fluctuations in orthorhombic 3$d^1$ perovskites
• Mutual Experimental and Theoretical Validation of Bulk Photoemission Spectra of Sr1-xCaxVO3
• How chemistry controls electron localization in 3d1 perovskites: A Wannier-function study
• Comparative study of correlation effects in CaVO3 and SrVO3
• Direct observation of the mass renormalization in SrVO${}_3$ by angle resolved photoemission spectroscopy
• Bulk and surface-sensitive high-resolution photoemission study of Mott-Hubbard systems SrVO${}_3$ and CaVO${}_3$
• Photoemission Spectral Weight Transfer and Mass Renormalization in the Fermi-Liquid System La${}_{1-x}$Sr${}_x$TiO${}_{3+y/2}$

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