Doped graphane: a prototype high-Tc electron-phonon superconductor
arXiv:1002.0653 · doi:10.1103/PhysRevLett.105.037002
Abstract
We show by first-principles calculations that p-doped graphane is a conventional superconductor with a critical temperature (Tc) above the boiling point of liquid nitrogen. The unique strength of the chemical bonds between carbon atoms and the large density of electronic states at the Fermi energy arising from the reduced dimensionality synergetically push Tc above 90K, and give rise to large Kohn anomalies in the optical phonon dispersions. As evidence of graphane was recently reported, and doping of related materials such as graphene, diamond and carbon nanostructures is well established, superconducting graphane may be feasible.
6 pages, 4 figures
References in corpus (13)
- Quantum ESPRESSO: a modular and open-source software project for quantum simulations of materials
- Two Dimensional Atomic Crystals
- Control of graphene's properties by reversible hydrogenation
- Electrochemically Top Gated Graphene: Monitoring Dopants by Raman Scattering
- Graphane: a two-dimensional hydrocarbon
- Edge-functionalized and substitutional doped graphene nanoribbons: electronic and spin properties
- Atomic Hole Doping of Graphene
- Three-dimensional MgB-type superconductivity in hole-doped diamond
- Origin of Superconductivity in Boron-doped Diamond
- Electron-Phonon Interactions in Graphene, Bilayer Graphene, and Graphite
- Giant non-adiabatic effects in layer metals: Raman spectra of intercalated graphite explained
- Prediction of superconducting properties of CaB2 using anisotropic Eliashberg theory
- Possibility of superconductivity in graphite intercalated with alkaline earths investigated with density functional theory
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