Calorimetric Evidence for a Fulde-Ferrell-Larkin-Ovchinnikov Superconducting State in the Layered Organic Superconductor κ_2_2$
arXiv:0706.3584 · doi:10.1103/PhysRevLett.99.187002
Abstract
The specific heat of the layered organic superconductor -% (BEDT-TTF)Cu(NCS), where BEDT-TTF is bisethylenedithio-% tetrathiafulvalene, has been studied in magnetic fields up to 28 T applied perpendicular and parallel to the superconducting layers. In parallel fields above 21 T, the superconducting transition becomes first order, which signals that the Pauli-limiting field is reached. Instead of saturating at this field value, the upper critical field increases sharply and a second first-order transition line appears within the superconducting phase. Our results give strong evidence that the phase, which separates the homogeneous superconducting state from the normal state is a realization of a Fulde-Ferrell-Larkin-Ovchinnikov state.
4pages, 3 figures
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