Structural and magnetic aspects of the metal insulator transition in Ca${}_{2-x}$Sr${}_x$RuO${}_4$

Abstract

The phase diagram of Ca${}_{2-x}$Sr${}_x$RuO${}_4$ has been studied by neutron diffraction on powder and single-crystalline samples. The experiments reveal antiferromagnetic order and structural distortions characterized by tilts and rotations of the RuO${}_6$-octahedra. There is strong evidence that the structural details of the isovalent samples tune the magnetic as well as the electronic behavior. In particular we observe for low Sr-concentration a metal insulator transition associated with a structural change and magnetic ordering.