Orbitally selective breakdown of Fermi liquid quasiparticles in Ca${}_{1.8}$Sr${}_{0.2}$RuO${}_4$

Abstract

We present a comprehensive angle-resolved photoemission spectroscopy study of Ca${}_{1.8}$Sr${}_{0.2}$RuO${}_4$. Four distinct bands are revealed and along the Ru-O bond direction their orbital characters are identified through a light polarization analysis and comparison to dynamical mean-field theory calculations. Bands assigned to $d_{xz},d_{yz}$ orbitals display Fermi liquid behavior with fourfold quasiparticle mass renormalization. Extremely heavy fermions - associated with a predominantly $d_{xy}$ band character - are shown to display non-Fermi-liquid behavior. We thus demonstrate that Ca${}_{1.8}$Sr${}_{0.2}$RuO${}_4$ is a hybrid metal with an orbitally selective Fermi liquid quasiparticle breakdown.

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• Oxide Fermi liquid universality revealed by electron spectroscopy
• Tunable electronic and magnetic phases in layered ruthenates: SrRuO3-SrTiO3 heterostructure upon strain
• Entropy and specific heat of the infinite-dimensional three-orbital Hubbard model
• Orbital-selective metal skin induced by alkali-metal-dosing Mott-insulating Ca${}_2$RuO${}_4$
• Orbitally-selective Breakdown of the Fermi Liquid and Simultaneous Enhancement of Metallic and Insulating States in Correlated Multi-band Systems with Spin-orbit Coupling
• Fragility of Topology under Electronic Correlations in Iron Chalcogenides
• Universal size-dependent nonlinear charge transport in single crystals of the Mott insulator Ca${}_2$RuO${}_4$
• Strain Engineering of van Hove Singularity and Coupled Itinerant Ferromagnetism in Quasi-2D Oxide Superlattices
• Hund's metallicity enhanced by van Hove singularity in cubic perovskite systems