Field-tuning of ultrafast magnetization fluctuations in Sm${}_{0.7}$Er${}_{0.3}$FeO${}_3$

Abstract

The properties of spin fluctuations in antiferromagnets are largely unexplored, in particular at ultrafast timescales. Here, we employ femtosecond noise correlation spectroscopy (FemNoC) to experimentally study magnetization fluctuations in the canted antiferromagnet Sm${}_{0.7}$Er${}_{0.3}$FeO${}_3$ across its spin reorientation transition and under external magnetic fields. By comparing our measurements to atomistic spin noise and Monte Carlo simulations, we find that the amplitude of the spin noise is governed by the free energy, with stronger fluctuations in regions where the potential landscape softens. We furthermore demonstrate that external magnetic fields suppress spin fluctuations and enhance the quasi-ferromagnetic magnon frequency by effectively stiffening the potential. These results highlight an effective route for tuning ultrafast magnetization fluctuations via external parameters.

11 pages, 10 figures

References in corpus (5)

• Subcycle Quantum Electrodynamics
• Spin canting in nonlinear terahertz magnon dynamics revealed by magnetorefractive probing in orthoferrite
• Ultrafast spontaneous spin switching in an antiferromagnet
• Subharmonic lock-in detection and its optimisation for femtosecond noise correlation spectroscopy
• Quantifying the amplitudes of ultrafast magnetization fluctuations in Sm${}_{0.7}$Er${}_{0.3}$FeO${}_3$ using femtosecond noise correlation spectroscopy