Simulating Chemistry on Bosonic Quantum Devices
arXiv:2404.10214 · doi:10.1021/acs.jctc.4c00544
Abstract
Bosonic quantum devices offer a novel approach to realize quantum computations, where the quantum two-level system (qubit) is replaced with the quantum (an)harmonic oscillator (qumode) as the fundamental building block of the quantum simulator. The simulation of chemical structure and dynamics can then be achieved by representing or mapping the system Hamiltonians in terms of bosonic operators. In this perspective, we review recent progress and future potential of using bosonic quantum devices for addressing a wide range of challenging chemical problems, including the calculation of molecular vibronic spectra, the simulation of gas-phase and solution-phase adiabatic and nonadiabatic chemical dynamics, the efficient solution of molecular graph theory problems, and the calculations of electronic structure.
40 pages including references, 13 figures, revised
References in corpus (76)
- A variational eigenvalue solver on a quantum processor
- Quantum information with continuous variables
- Gaussian Quantum Information
- Charge insensitive qubit design derived from the Cooper pair box
- Circuit Quantum Electrodynamics
- Dynamical Decoupling of Open Quantum Systems
- Quantum computational chemistry
- Manipulating the Quantum State of an Electrical Circuit
- Quantum Chemistry in the Age of Quantum Computing
- Trapped-Ion Quantum Computing: Progress and Challenges
- An adaptive variational algorithm for exact molecular simulations on a quantum computer
- Quantum algorithms for quantum chemistry and quantum materials science
- Hartree-Fock on a superconducting qubit quantum computer
- Determining eigenstates and thermal states on a quantum computer using quantum imaginary time evolution
- Reconstruction of non-classical cavity field states with snapshots of their decoherence
- Roads towards fault-tolerant universal quantum computation
- Variational ansatz-based quantum simulation of imaginary time evolution
- Perspective: Numerically "exact" approach to open quantum dynamics: The hierarchical equations of motion (HEOM)
- Gaussian Boson Sampling
- Qudits and high-dimensional quantum computing
- Quantum Phase Transitions and Bipartite Entanglement
- Planar Superconducting Resonators with Internal Quality Factors above One Million
- Encoding a qubit in a trapped-ion mechanical oscillator
- A quantum memory with near-millisecond coherence in circuit QED
- Boson Sampling for Molecular Vibronic Spectra
- Strawberry Fields: A Software Platform for Photonic Quantum Computing
- Demonstration of fidelity improvement using dynamical decoupling with superconducting qubits
- Deterministic creation of entangled atom-light Schrödinger-cat states
- Emerging quantum computing algorithms for quantum chemistry
- Fast Universal Control of an Oscillator with Weak Dispersive Coupling to a Qubit
- Superconducting Qubits: A Short Review
- Suppression of crosstalk in superconducting qubits using dynamical decoupling
- Molecular Docking with Gaussian Boson Sampling
- Efficient multiphoton sampling of molecular vibronic spectra on a superconducting bosonic processor
- Dynamical decoupling for superconducting qubits: a performance survey
- Focus beyond quadratic speedups for error-corrected quantum advantage
- Quantum Simulation of Open Quantum Systems Using a Unitary Decomposition of Operators
- Quantum Solver of Contracted Eigenvalue Equations for Scalable Molecular Simulations on Quantum Computing Devices
- Excited-state quantum phase transitions
- Calculating the Thermal Rate Constant with Exponential Speed-Up on a Quantum Computer
- Applications of Near-Term Photonic Quantum Computers: Software and Algorithms
- Combining dynamical decoupling with fault-tolerant quantum computation
- Kerr-free three-wave mixing in superconducting quantum circuits
- A perspective on hybrid quantum opto- and electromechanical systems
- Generalized Quantum Master Equations In and Out of Equilibrium: When Can One Win?
- Universal Gate Set for Continuous-Variable Quantum Computation with Microwave Circuits
- Approximate but Accurate Quantum Dynamics from the Mori Formalism: I. Nonequilibrium Dynamics
- An Introduction to the Transmon Qubit for Electromagnetic Engineers
- Demonstration of algorithmic quantum speedup
- Quantum Phase Estimation with Time-Frequency Qudits in a Single Photon
- Quantum approximate optimization with Gaussian boson sampling
- Efficient construction of generalized master equation memory kernels for multi-state systems from nonadiabatic quantum-classical dynamics
- Universal control of a bosonic mode via drive-activated native cubic interactions
- Hierarchical equations of motion approach to hybrid fermionic and bosonic environments: Matrix product state formulation in twin space
- Simulating Open Quantum System Dynamics on NISQ Computers with Generalized Quantum Master Equations
- Franck-Condon factors by counting perfect matchings of graphs with loops
- Efficient low temperature simulations for fermionic reservoirs with the hierarchical equations of motion method: Application to the Anderson impurity model
- Tensor-Train Thermo-Field Memory Kernels for Generalized Quantum Master Equations
- Spectral kissing and its dynamical consequences in the squeeze-driven Kerr oscillator
- Approximate but accurate quantum dynamics from the Mori formalism: II. Equilibrium correlation functions
- Observation of wave-packet branching through an engineered conical intersection
- Excited state quantum phase transitions in the bending spectra of molecules
- Exact operator bosonization of finite number of fermions in one space dimension
- Calculation of Transition State Energies in the HCN-HNC Isomerization with an Algebraic Model
- Quantum tunneling and level crossings in the squeeze-driven Kerr oscillator
- Double-excitation manifold's effect on exciton transfer dynamics and the efficiency of coherent light harvesting
- Shaping photons: quantum computation with bosonic cQED
- Entanglement in Graph States and its Applications
- Symmetries of the squeeze-driven Kerr oscillator
- Variational quantum iterative power algorithms for global optimization
- Efficient formulation of multitime generalized quantum master equations: Taming the cost of simulating 2D spectra
- Note: Nonuniqueness of generalized quantum master equations for a single observable
- Quantum-inspired classical algorithm for graph problems by Gaussian boson sampling
- A driven quantum superconducting circuit with multiple tunable degeneracies
- Heterogeneous Multipartite Entanglement Purification for Size-Constrained Quantum Devices
- Bosonic Qiskit
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- Hybrid Oscillator-Qubit Quantum Processors: Instruction Set Architectures, Abstract Machine Models, and Applications
- Simulating Non-Markovian Quantum Dynamics on NISQ Computers Using the Hierarchical Equations of Motion
- A Roadmap for Simulating Chemical Dynamics on a Parametrically Driven Bosonic Quantum Device
- Simulating Vibrational Dynamics on Bosonic Quantum Devices
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- Quantum squeezing amplification with a weak Kerr nonlinear oscillator
- Adaptive variational quantum computing approaches for Green's functions and nonlinear susceptibilities
- A Computational Framework for Simulations of Dissipative Non-Adiabatic Dynamics on Hybrid Oscillator-Qubit Quantum Devices
- Unitary death of Schrödinger's cat
- Simulating electronic structure on bosonic quantum computers
- Quantum Computing Beyond Ground State Electronic Structure: A Review of Progress Toward Quantum Chemistry Out of the Ground State
- Quantum-computing within a bosonic context: Assessing finite basis effects on prototypical vibrational Hamiltonian spectra
- Phase transitions, symmetries, and tunneling in Kerr parametric oscillators
- Quantum Simulation of Charge and Exciton Transfer in Multi-mode Models using Engineered Reservoirs
- Delocalized Excitation Transfer in Open Quantum Systems with Long-Range Interactions
- Quantum Simulation of Two-Level -Symmetric Systems Using Hermitian Hamiltonians
- Digital quantum simulation of bosonic systems and quantum complementarity
- Degeneracy beyond the parity-symmetry protection in one-dimensional spinless models: The parity-violating Kerr parametric oscillator