Boson Sampling for Molecular Vibronic Spectra
arXiv:1412.8427 · doi:10.1038/nphoton.2015.153
Abstract
Quantum computers are expected to be more efficient in performing certain computations than any classical machine. Unfortunately, the technological challenges associated with building a full-scale quantum computer have not yet allowed the experimental verification of such an expectation. Recently, boson sampling has emerged as a problem that is suspected to be intractable on any classical computer, but efficiently implementable with a linear quantum optical setup. Therefore, boson sampling may offer an experimentally realizable challenge to the Extended Church-Turing thesis and this remarkable possibility motivated much of the interest around boson sampling, at least in relation to complexity-theoretic questions. In this work, we show that the successful development of a boson sampling apparatus would not only answer such inquiries, but also yield a practical tool for difficult molecular computations. Specifically, we show that a boson sampling device with a modified input state can be used to generate molecular vibronic spectra, including complicated effects such as Duschinsky rotations.
10 pages, 6 figures
References in corpus (7)
- Simulated Quantum Computation of Molecular Energies
- Photonic Boson Sampling in a Tunable Circuit
- Simulating chemistry using quantum computers
- Chemical Basis of Trotter-Suzuki Errors in Quantum Chemistry Simulation
- Demonstration of deterministic and high fidelity squeezing of quantum information
- Universal optical amplification without nonlinearity
- Sampling arbitrary photon-added or photon-subtracted squeezed states is in the same complexity class as boson sampling
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