Delocalized Excitation Transfer in Open Quantum Systems with Long-Range Interactions
arXiv:2502.04383 · doi:10.1103/bxwl-sbsn
Abstract
The interplay between coherence and system-environment interactions is at the basis of a wide range of phenomena, from quantum information processing to charge and energy transfer in molecular systems, biomolecules, and photochemical materials. In this work, we use a Frenkel exciton model with long-range interacting qubits coupled to a damped collective bosonic mode to investigate vibrationally assisted transfer processes in donor-acceptor systems featuring internal substructures analogous to light-harvesting complexes. We find that certain delocalized excitonic states maximize the transfer rate and that the entanglement is preserved during the dissipative transfer over a wide range of parameters. We investigate the reduction in transfer caused by static disorder, white noise, and finite temperature and study how transfer efficiency scales as a function of the number of dimerized monomers and the component number of each monomer, finding which excitonic states lead to optimal transfer. Finally, we provide a realistic experimental setting to realize this model in analog trapped-ion quantum simulators. Analog quantum simulation of systems comprising many and increasingly complex monomers could offer valuable insights into the design of light-harvesting materials, particularly in the non-perturbative intermediate parameter regime examined in this study, where classical simulation methods are resource-intensive.
18 pages, 6 figures, Appendices included
References in corpus (61)
- Three qubits can be entangled in two inequivalent ways
- Distributed Entanglement
- Quantum States and Phases in Driven Open Quantum Systems with Cold Atoms
- Environment-Assisted Quantum Walks in Photosynthetic Energy Transfer
- Dephasing assisted transport: Quantum networks and biomolecules
- Programmable Quantum Simulations of Spin Systems with Trapped Ions
- Highly efficient energy excitation transfer in light-harvesting complexes: The fundamental role of noise-assisted transport
- Quantum harmonic oscillator state synthesis by reservoir engineering
- Non-perturbative treatment of non-Markovian dynamics of open quantum systems
- Engineered Dissipation for Quantum Information Science
- Delocalized excitons in natural light harvesting complexes
- Non-Markovianity assisted Steady State Entanglement
- Unconventional magnetism via optical pumping of interacting spin systems
- Effective Spin Quantum Phases in Systems of Trapped Ions
- Environment-assisted quantum transport in a 10-qubit network
- Quantum Simulation of Generic Many-Body Open System Dynamics Using Classical Noise
- Mesoscopic Entanglement Induced by Spontaneous Emission in Solid-State Quantum Optics
- Large Scale Quantum Computation in an Anharmonic Linear Ion Trap
- Dissipative Floquet Dynamics: from Steady State to Measurement Induced Criticality in Trapped-ion Chains
- Towards analog quantum simulations of lattice gauge theories with trapped ions
- Origin of long-lived oscillations in 2D-spectra of a Quantum Vibronic Model: Electronic vs Vibrational coherence
- Efficient quantum algorithms for and states, and implementation on the IBM quantum computer
- Experimental Realization of a Quantum Integer-Spin Chain with Controllable Interactions
- Diverging equilibration times in long-range quantum spin models
- Studying Light-Harvesting Models with Superconducting Circuits
- Impact of environmentally induced fluctuations on quantum mechanically mixed electronic and vibrational pigment states in photosynthetic energy transfer and 2D electronic spectra
- Optical pumping into many-body entanglement
- When polarons meet polaritons: Exciton-vibration interactions in organic molecules strongly coupled to confined light fields
- Dissipation-assisted matrix product factorization
- Engineering vibrationally-assisted energy transfer in a trapped-ion quantum simulator
- Emergent dark states from superradiant dynamics in multilevel atoms in a cavity
- Dissipative quantum control of a spin chain
- Direct observation of geometric phase in dynamics around a conical intersection
- Analog quantum simulation of chemical dynamics
- Cross-Kerr nonlinearity for phonon counting
- Signaling and Scrambling with Strongly Long-Range Interactions
- The squeezed Kerr oscillator: spectral kissing and phase-flip robustness
- Interplay of Soundcone and Supersonic Propagation in Lattice Models with Power Law Interactions
- Optimal State Transfer and Entanglement Generation in Power-law Interacting Systems
- Simulating Chemistry on Bosonic Quantum Devices
- Quantum Simulation of Spin-Boson Models with Structured Bath
- Seeking a quantum advantage with trapped-ion quantum simulations of condensed-phase chemical dynamics
- Environment-assisted quantum transport and mobility edges
- Trapped-Ion Quantum Simulation of Electron Transfer Models with Tunable Dissipation
- Lieb-Robinson bounds for open quantum systems with long-ranged interactions
- Experimental Quantum Simulation of Chemical Dynamics
- Continuously parametrized quantum simulation of molecular electron transfer reactions
- Controlling Matter Phases beyond Markov
- Unraveling excitation energy transfer assisted by collective behaviors of vibrations
- Constructing the spin-1 Haldane phase on a qudit quantum processor
- Interplay of vibration- and environment-assisted energy transfer
- Quantum Simulation of Polarized Light-induced Electron Transfer with A Trapped-ion Qutrit System
- A Roadmap for Simulating Chemical Dynamics on a Parametrically Driven Bosonic Quantum Device
- Indirect Cooling of Weakly Coupled Trapped-Ion Mechanical Oscillators
- Spectral theory of non-Markovian dissipative phase transitions
- Sideband thermometry of ion crystals
- Driven-dissipative four-mode squeezing of multilevel atoms in an optical cavity
- Accelerating two-dimensional electronic spectroscopy simulations with a probe qubit protocol
- Time optimal quantum state transfer in a fully-connected quantum computer
- Enhancement of vibrationally assisted energy transfer by proximity to exceptional points, probed by fluorescence-detected vibrational spectroscopy
- Optimisation of ultrafast singlet fission in 1D rings towards unit efficiency