Dirac Cones and Room Temperature Polariton Lasing Evidenced in an Organic Honeycomb Lattice
arXiv:2401.10126 · doi:10.1002/advs.202400672
Abstract
Artificial one- and two-dimensional lattices have emerged as a powerful platform for the emulation of lattice Hamiltonians, the fundamental study of collective many-body effects, and phenomena arising from non-trivial topology. Exciton-polaritons, bosonic part-light and part-matter quasiparticles, combine pronounced nonlinearities with the possibility of on-chip implementation. In this context, organic semiconductors embedded in microcavities have proven to be versatile candidates to study nonlinear many-body physics and bosonic condensation, and in contrast to most inorganic systems, they allow the use at ambient conditions since they host ultra-stable Frenkel excitons. We implement a well-controlled, high-quality optical lattice that accommodates light-matter quasiparticles. The realized polariton graphene presents with excellent cavity quality factors, showing distinct signatures of Dirac cone and flatband dispersions as well as polariton lasing at room temperature. This is realized by filling coupled dielectric microcavities with the fluorescent protein mCherry. We demonstrate the emergence of a coherent polariton condensate at ambient conditions, taking advantage of coupling conditions as precise and controllable as in state-of-the-art inorganic semiconductor-based systems, without the limitations of e.g. lattice matching in epitaxial growth. This progress allows straightforward extension to more complex systems, such as the study of topological phenomena in two-dimensional lattices including topological lasers and non-Hermitian optics.
28 pages, 9 figures
References in corpus (11)
- The electronic properties of graphene
- Many-Body Physics with Ultracold Gases
- Substrate-induced band gap opening in epitaxial graphene
- Quantum fluids of light
- Strong light-matter coupling in two-dimensional atomic crystals
- Observation of Superfluidity of Polaritons in Semiconductor Microcavities
- Tools for quantum simulation with ultracold atoms in optical lattices
- Polariton condensation in - and -flatbands in a two-dimensional Lieb lattice
- Electrically tunable Berry curvature and strong light-matter coupling in birefringent perovskite microcavities at room temperature
- Fully tunable exciton-polaritons emerging from WS monolayer excitons in an optical lattice at room temperature
- Dirac Cones and Room Temperature Polariton Lasing Evidenced in an Organic Honeycomb Lattice
Cited by in corpus (4)
- In-situ tunable, room-temperature polariton condensation in individual states of a 1D topological lattice
- Dirac Cones and Room Temperature Polariton Lasing Evidenced in an Organic Honeycomb Lattice
- Enwrapped Perylene Bisimide Enables Room Temperature Polariton Lasing and Photonic Lattices
- Polaritonic Machine Learning for Graph-based Data Analysis