Excitonic interplay between surface polar III-nitride quantum wells and MoS monolayer
arXiv:2308.10687 · doi:10.1021/acs.nanolett.4c02259
Abstract
III-nitride wide bandgap semiconductors exhibit large exciton binding energies, preserving strong excitonic effects at room temperature. On the other hand, semiconducting two-dimensional (2D) materials, including MoS, also exhibit strong excitonic effects, attributed to enhanced Coulomb interactions. This study investigates excitonic interactions between surface GaN quantum well (QW) and 2D MoS in van der Waals heterostructures by varying the spacing between these two excitonic systems. Optical property investigation first demonstrates the effective passivation of defect states at the GaN surface through MoS coating. Furthermore, a strong interplay is observed between MoS monolayers and GaN QW excitonic transitions. This highlights the interest of the 2D material/III-nitride QW system to study near-field interactions, such as Förster resonance energy transfer, which could open up novel optoelectronic devices based on such hybrid excitonic structures.
arXiv commentCorrected error bars in Fig. 3
References in corpus (10)
- Electric Field Effect in Atomically Thin Carbon Films
- Mixed-Dimensional van der Waals Heterostructures
- Rapid and reliable thickness identification of two-dimensional nanosheets using optical microscopy
- Macroscopic polarization and band offsets at nitride heterojunctions
- Quantitative Raman Spectrum and Reliable Thickness Identification for Atomic Layers on Insulating Substrates
- Spatially resolved optical absorption spectroscopy of single- and few-layer MoS2 by hyperspectral imaging
- Electric field induced strong enhancement of electroluminescence in multi-Layer MoS2
- Interface Dipole and Band Bending in Hybrid p-n Heterojunction MoS2/GaN(0001)
- Interlayer Charge Transfer and Defect Creation in Type I van der Waals Heterostructures
- Quenching of the luminescence intensity of GaN nanowires under electron beam exposure: Impact of C adsorption on the exciton lifetime