Ionic Coherence in Resonant Above-Threshold Attosecond Ionization Spectroscopy

Abstract

The ionization of atoms with sequences of attosecond pulses gives rise to excited ionic states that are entangled with the emitted photoelectron. Still, the ionic ensemble preserves some coherence that can be controlled through the laser parameters. In helium, control of the $2s/2p$ He${}^{+}$ coherence is mediated by the autoionizing states below the $N=2$ threshold [Phys. Rev. Res. {\bf 3}, 023233 (2021)]. In the present work we study the role of the resonances both below and above the $N=3$ threshold on the coherence of the $N=3$ He${}^{+}$ ion, in the attosecond pump-probe ionization of the helium atom, which we simulate using the newstock \emph{ab initio} code. Due to the fine-structure splitting of the N=3 He${}^{+}$ level, the ionic dipole beats on a picosecond timescale. We show how, from the dipole beating, it is possible to reconstruct the polarization of the ion at its inception.

arXiv comment13 pages, 9 figures

References in corpus (13)

• The Magnus expansion and some of its applications
• CODATA Recommended Values of the Fundamental Physical Constants: 2014
• Attosecond physics at the nanoscale
• Attosecond dynamics through a Fano resonance: Monitoring the birth of a photoelectron
• Phase measurement of a Fano window resonance using tunable attosecond pulses
• Decoherence in Attosecond Photoionization
• The Multi-Configurational Hartree-Fock close-coupling ansatz: application to Argon photoionization cross section and delays
• Modulation of attosecond beating in resonant two-photon ionization
• Photoionization of helium by attosecond pulses: extraction of spectra from correlated wave functions
• Ionization branching ratio control with a resonance attosecond clock
• Can strong-field ionization prepare attosecond dynamics?
• Autoionizing Polaritons in Attosecond Atomic Ionization
• Coherent control of an Helium-Ion ensemble

Cited by in corpus (1)

• Entanglement Transfer in a Composite Electron-Ion-Photon System