Attosecond physics at the nanoscale
arXiv:1607.01480 · doi:10.1088/1361-6633/aa574e
Abstract
Recently two emerging areas of research, attosecond and nanoscale physics, have started to come together. Attosecond physics deals with phenomena occurring when ultrashort laser pulses, with duration on the femto- and sub-femtosecond time scales, interact with atoms, molecules or solids. The laser-induced electron dynamics occurs natively on a timescale down to a few hundred or even tens of attoseconds, which is comparable with the optical field. On the other hand, the second branch involves the manipulation and engineering of mesoscopic systems, such as solids, metals and dielectrics, with nanometric precision. Although nano-engineering is a vast and well-established research field on its own, the merger with intense laser physics is relatively recent. In this article we present a comprehensive experimental and theoretical overview of physics that takes place when short and intense laser pulses interact with nanosystems, such as metallic and dielectric nanostructures. In particular we elucidate how the spatially inhomogeneous laser induced fields at a nanometer scale modify the laser-driven electron dynamics. Consequently, this has important impact on pivotal processes such as ATI and HHG. The deep understanding of the coupled dynamics between these spatially inhomogeneous fields and matter configures a promising way to new avenues of research and applications. Thanks to the maturity that attosecond physics has reached, together with the tremendous advance in material engineering and manipulation techniques, the age of atto-nano physics has begun, but it is in the initial stage. We present thus some of the open questions, challenges and prospects for experimental confirmation of theoretical predictions, as well as experiments aimed at characterizing the induced fields and the unique electron dynamics initiated by them with high temporal and spatial resolution.
Invited Review ROPP, 50 pages, 38 figures
References in corpus (55)
- Sub-cycle control of terahertz high-harmonic generation by dynamical Bloch oscillations
- Attosecond control of electrons emitted from a nanoscale metal tip
- A Femtosecond Nanometer Free Electron Source
- Attosecond double-slit experiment
- A spatially and temporally localized sub-laser-cycle electron source
- Strong-field above-threshold photoemission from sharp metal tips
- Simultaneous compression and characterization of ultrashort laser pulses using chirped mirrors and glass wedges
- Carrier-envelope phase effects on the strong-field photoemission of electrons from metallic nanostructures
- Imaging an aligned polyatomic molecule with laser-induced electron diffraction
- Laser-induced ultrafast electron emission from a field emission tip
- High-order harmonic generation from inhomogeneous fields
- Theory of plasmon-enhanced high-harmonic generation in the vicinity of metal nanostructures in noble gases
- Highly coherent electron beam from a laser-triggered tungsten needle tip
- Energy-dependent photoemission delays from noble metal surfaces by attosecond interferometry
- Mechanism of Laser-induced Field Emission
- Beyond Carbon K-edge harmonic emission using spatial and temporal synthesized laser field
- A nanofocused plasmon-driven sub-10 femtosecond electron point source
- Femtosecond electrons probing currents and atomic structure in nanomaterials
- Optical Control of Field-Emission Sites by Femtosecond Laser Pulses
- A macroscopic test of the Aharonov-Bohm effect
- Quantum-orbit analysis of high-order harmonic generation by resonant plasmon field enhancement
- Steering proton migration in hydrocarbons using intense few-cycle laser fields
- Simulation of attosecond streaking of electrons emitted from a tungsten surface
- Probing of optical near-fields by electron rescattering on the 1 nm scale
- High-order harmonic generation by enhanced plasmonic near-fields in metal nanoparticules
- Electron rescattering at metal nanotips induced by ultrashort laser pulses
- Streaking and Wigner time delays in photoemission from atoms and surfaces
- Attosecond nanoscale near-field sampling
- Large optical field enhancement for nanotips with large opening angles
- A tip-based source of femtosecond electron pulses at 30keV
- Laser-induced Field Emission from Tungsten Tip: Optical Control of Emission Sites and Emission Process
- Attosecond nanoplasmonic streaking of localized fields near metal nanospheres
- Ultrafast laser-triggered emission from hafnium carbide tips
- High order harmonic generation in noble gases using plasmonic field enhancement
- Temporal and spectral disentanglement of laser-driven electron tunneling emission from a solid
- Above threshold ionization by few-cycle spatially inhomogeneous fields
- Electron momentum distributions and photoelectron spectra of atoms driven by intense spatially inhomogeneous field
- Quantum-orbit analysis of above threshold ionization by intense spatially inhomogeneous field
- Nonsequential Double Recombination in Intense Laser Fields
- A nanoscale vacuum-tube diode triggered by few-cycle laser pulses
- Attosecond spectroscopy of solids: streaking phase shift due to lattice scattering
- Laser-induced electron emission from a tungsten nanotip: identifying above threshold photoemission using energy-resolved laser power dependencies
- High-order harmonic generation from Rydberg atoms driven by plasmonic-enhanced laser fields
- Generation and Bistability of a Waveguide Nanoplasma Observed by Enhanced Extreme-Ultraviolet Fluorescence
- Carrier-envelope phase stability of hollow-fibers used for high-energy, few-cycle pulse generation
- ClassSTRONG: Classical simulations of Strong Field processes
- High-order harmonic generation driven by metal nanotip photoemission: theory and simulations
- Four-state rock-paper-scissors games on constrained Newman-Watts networks
- Attosecond Photoscopy of Plasmonic Excitations
- Estimating the plasmonic field enhancement using high-order harmonic generation: The role of inhomogeneity of the fields
- Signatures of double-electron re-combination in high-order harmonic generation driven by spatially inhomogeneous fields
- Numerical studies of light-matter interaction driven by plasmonic fields: the velocity gauge
- Coherent XUV generation driven by sharp metal tips photoemission
- Different time scales in plasmonically enhanced high-order harmonic generation
- Ultrafast time resolved photo-electric emission
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- Tunable Isolated Attosecond X-ray Pulses with Gigawatt Peak Power from a Free-Electron Laser
- Strong-field Phenomena in Periodic Systems
- Symphony on Strong Field Approximation
- Wannier-Bloch approach to localization in high harmonics generation in solids
- On-chip sampling of optical fields with attosecond resolution
- Relativistic near-single-cycle optics at 1 kHz
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- High-purity free-electron momentum states prepared by three-dimensional optical phase modulation
- Attosecond electron microscopy by free-electron homodyne detection
- Coulomb-correlated electron number states in a transmission electron microscope beam
- Sub-cycle quantum electrodynamics in strongly laser-driven semiconductors
- Coherent two-dimensional multiphoton photoelectron spectroscopy of metal surfaces
- Strong laser physics, non-classical light states and quantum information science
- Implications of gauge freedom for nonrelativistic quantum electrodynamics
- Generating high-order optical and spin harmonics from ferromagnetic monolayers
- Light Phase Detection with On-Chip Petahertz Electronic Networks
- Strong laser fields and their power to generate controllable high-photon-number coherent-state superpositions
- High-harmonic generation in quantum spin systems
- Few-cycle pulse generation by double-stage hybrid multi-pass multi-plate nonlinear pulse compression
- High-order harmonic generation in atomic and molecular systems
- Improved one-dimensional model potentials for strong-field simulations
- High-order above-threshold photoemission from nanotips controlled with two-color laser fields
- Adiabaticity parameters for the categorization of light-matter interaction -- from weak to strong driving
- Tomography of asymmetric molecular orbitals with one-color inhomogeneous field
- Ab initio study of time-dependent dynamics in strong-field triple ionization
- Attosecond Ionization Time Delays in Strong-Field Physics
- Emergence of a higher energy structure in strong field ionization with inhomogeneous electric fields
- Laser control of magnonic topological phases in antiferromagnets
- Controlling polarization of attosecond pulses with plasmonic-enhanced bichromatic counter-rotating circularly polarised fields
- Simultaneous control of harmonic yield and energy cutoff of high-harmonic generation using seeded plasmonic-enhanced fields
- Protein Structured Reservoir computing for Spike-based Pattern Recognition
- Structured squeezed light allows for high-harmonic generation in classical forbidden geometries
- Multielectron interference of intraband harmonics in solids
- Ultrafast Laser Driven Many-Body Dynamics and Kondo Coherence Collapse
- Imaging the source of high-harmonics generated in atomic gas media
- Density-based one-dimensional model potentials for strong-field simulations in , and
- Lightwave-Electronic Harmonic Frequency Mixing
- Phase matching effects in high harmonic generation at the nanometer scale
- Optical Distinguishability of Mott Insulators in Time vs Frequency Domain
- Impact of DC bias on Weak Optical-Field-Driven Electron Emission in Nano-Vacuum-Gap Detectors
- Quantum Nanophotonics with Energetic Particles:X-rays and Free Electrons
- Attoscience in Phase Space
- Analytical approximations for the higher energy structure in strong field ionization with inhomogeneous electric fields
- Optomagnonic Barnett effect
- One-dimensional model potentials optimized for the calculation of the HHG spectrum
- Light-dressed states under intense optical near fields
- Analog simulation of high harmonic generation in atoms
- Ionic Coherence in Resonant Above-Threshold Attosecond Ionization Spectroscopy
- Controlling quantum effects in enhanced strong-field ionisation with machine-learning techniques
- Tuning the electronic band structure of metal surfaces for enhancing high-order harmonic generation
- Double-electron ionization driven by inhomogeneous fields
- Optomagnonic Josephson effect in antiferromagnets
- Spin-valley dynamics of electrically driven ambipolar carbon-nanotube quantum dots
- Exploring Spin Symmetry-Breaking Effects for Static Field Ionization of Atoms: Is There an Analog to the Coulson-Fischer Point in Bond Dissociation?
- Coherent control of an Helium-Ion ensemble
- Photon pumping, photodissociation and dissipation at interplay for the fluorescence of a molecule in a cavity
- A DFT-based Tight-Binding Approach to the Self-consistent Description of Molecule Metal-Nanoparticle Interactions
- First-principles method for nonlinear light propagation at oblique incidence
- Beyond Fowler-Nordheim model: Harmonic generation from metallic nano-structures
- Coherent Control of Relativistic Electron Dynamics in Plasma Nanophotonics
- Few-Photon Fluorescence from Ultracold Bosons in an Optical Cavity
- Optimal control of photoelectron emission by realistic waveforms
- Femtosecond pulse parameter estimation from photoelectron momenta using machine learning
- Generation of Super Intense Isolated Attosecond Pulses from Trapped Electrons in Metal Surfaces
- Broadband coherent XUV light from microbunching in an intense laser pulse
- Ultrafast optically induced tunneling in narrow metallic gaps from the time dependent density functional perspective
- Direct and alternating magnon spin currents across a junction interface irradiated by linearly polarized laser