Spectral function of the Heisenberg model on the triangular lattice
arXiv:2209.00739 · doi:10.1103/PhysRevB.107.165146
Abstract
Spectral probes, such as neutron scattering, are crucial for characterizing excitations in quantum many-body systems and the properties of quantum materials. Among the most elusive phases of matter are quantum spin liquids, which have no long-range order even at zero temperature and host exotic fractionalized excitations with non-trivial statistics. These phases can occur in frustrated quantum magnets, such as the paradigmatic Heisenberg model with nearest and next-nearest neighbor exchange interactions on the triangular lattice, the so-called model. In this work, we compute the spectral function using large scale matrix product state simulations across the three different phases of this model's phase diagram, including a quantum spin liquid phase at intermediate . Despite a plethora of theoretical and experimental studies, the exact nature of this phase is still contested, with the dominant candidates being a gapped , a gapless Dirac, and a spinon Fermi surface quantum spin liquid state. We find a V-shaped spectrum near the center of the Brillouin zone ( point), a key signature of a spinon Fermi surface, observed in prior neutron scattering experiments. However, we find a small gap near the point, ruling out such a phase. Furthermore, we find localized gapless excitations at the corner of the Brillouin zone boundary (K point) and the middle of the edge of the Brillouin zone boundary (M point), ruling out the gapped spin liquid phase. Our results imply that the intermediate spin liquid phase is a gapless Dirac spin liquid, and provide clear signatures to detect this phase in future neutron scattering experiments.
arXiv comment18 pages (8 figures)
References in corpus (145)
- The density-matrix renormalization group in the age of matrix product states
- Distributed Entanglement
- Quantum Spin Liquids
- Efficient simulation of one-dimensional quantum many-body systems
- Computational complexity and fundamental limitations to fermionic quantum Monte Carlo simulations
- Fractionalized excitations in the spin liquid state of a kagomé lattice antiferromagnet
- An Area Law for One Dimensional Quantum Systems
- Quantum Spin Liquids
- The ITensor Software Library for Tensor Network Calculations
- Time-dependent variational principle for quantum lattices
- Probing Topological Spin Liquids on a Programmable Quantum Simulator
- Matrix Product States and Projected Entangled Pair States: Concepts, Symmetries, and Theorems
- Unifying time evolution and optimization with matrix product states
- Time-evolution methods for matrix-product states
- Fisher information and multiparticle entanglement
- A Field Guide to Spin Liquids
- Quantum magnetism and criticality
- Long range Neel order in the triangular Heisenberg model
- Continuous excitations of the triangular-lattice quantum spin liquid YbMgGaO4
- Exact spectra, spin susceptibilities and order parameter of the quantum Heisenberg antiferromagnet on the triangular lattice
- Rare-earth triangular lattice spin liquid: a single-crystal study of YbMgGaO
- Evidence for a spinon Fermi surface in a triangular lattice quantum spin liquid candidate
- Theory of finite-entanglement scaling at one-dimensional quantum critical points
- Measuring multipartite entanglement via dynamic susceptibilities
- Neel order in square and triangular lattice Heisenberg models
- Gapless quantum spin liquid ground state in the two-dimensional spin-1/2 triangular antiferromagnet YbMgGaO
- Universality of Phase Transition Dynamics: Topological Defects from Symmetry Breaking
- Properties of an algebraic spin liquid on the kagome lattice
- Experimental Realization of Spin-1/2 Triangular-Lattice Heisenberg Antiferromagnet
- Spin liquid nature in the Heisenberg - triangular antiferromagnet
- Dynamics of Entanglement in One-Dimensional Spin Systems
- Spin liquid phase of the Heisenberg model on the triangular lattice
- Field-tunable quantum disordered ground state in the triangular lattice antiferromagnet NaYbO
- Algebraic spin liquid as the mother of many competing orders
- Spin Liquid States on the Triangular and Kagome Lattices: A Projective Symmetry Group Analysis of Schwinger Boson States
- Spin-waves in triangular lattice antiferromagnet: decays, spectrum renormalization, and singularities
- Magnetization Process and Collective Excitations in the S=1/2 Triangular-Lattice Heisenberg Antiferromagnet Ba3CoSb2O9
- SR evidence for the U(1) quantum spin liquid ground state in the triangular antiferromagnet YbMgGaO
- Post-Matrix Product State Methods: To tangent space and beyond
- Competing Spin Liquid States in the Spin- Heisenberg Model On Triangular Lattice
- Crystalline Electric Field Randomness in the Triangular Lattice Spin-Liquid YbMgGaO
- Tangent-space methods for uniform matrix product states
- Chiral spin liquid phase of the triangular lattice Hubbard model: a density matrix renormalization group study
- NaYbS - a new planar spin- triangular-lattice magnet and putative spin liquid
- Critical level crossings and gapless spin liquid in the square-lattice spin- - Heisenberg antiferromagnet
- Gapless spin-liquid state in the structurally disorder-free triangular antiferromagnet NaYbO
- Spin-glass ground state in a triangular-lattice compound YbZnGaO
- Anisotropic field-induced ordering in the triangular-lattice quantum spin liquid NaYbSe
- Anomalous dielectric response in the dimer Mott insulator -(BEDT-TTF)Cu(CN)
- Dirac Spin Liquid on the Spin-1/2 Triangular Heisenberg Antiferromagnet
- Excitation spectra of the spin-1/2 triangular-lattice Heisenberg antiferromagnet
- Studying quantum spin systems through entanglement estimators
- Field-induced instability of the quantum-spin-liquid ground state in the triangular-lattice compound NaYbO
- Time Dependent Variational Principle with Ancillary Krylov Subspace
- Absence of magnetic thermal conductivity in the quantum spin liquid candidate YbMgGaO4
- Static and Dynamical Properties of the Spin-1/2 Equilateral Triangular-Lattice Antiferromagnet BaCoSbO
- Crucial Role of Quantum Entanglement in Bulk Properties of Solids
- Chebyshev matrix product state approach for spectral functions
- Chiral Spin Liquid and Quantum Criticality in Extended Heisenberg Models on the Triangular Lattice
- Dynamical structure factor of triangular-lattice antiferromagnet
- Detection of Kardar-Parisi-Zhang hydrodynamics in a quantum Heisenberg spin- chain
- Nearly deconfined spinon excitations in the square-lattice spin-1/2 Heisenberg antiferromagnet
- Unifying Description of Competing Orders in Two Dimensional Quantum Magnets
- Divergence of the entanglement range in low dimensional quantum systems
- Anomalous Excitation Spectra of Frustrated Quantum Antiferromagnets
- Quantum spin liquid ground state in the disorder free triangular lattice NaYbS
- Lattice effects and entropy release at the low-temperature phase transition in the spin-liquid candidate -(BEDT-TTF)Cu(CN)
- The nature of spin excitations in the one-third magnetization plateau phase of BaCoSbO
- Global phase diagram and quantum spin liquids in spin-1/2 triangular antiferromagnet
- Spinon Fermi surface spin liquid in a triangular lattice antiferromagnet NaYbSe
- Magnon Decay in Noncollinear Quantum Antiferromagnets
- Flat spin wave dispersion in a triangular antiferromagnet
- Absence of charge order in the dimerized κ-phase BEDT-TTF salts
- Dynamical structure factor of the Heisenberg model on the triangular lattice: magnons, spinons, and gauge fields
- Spectral Functions with the Density Matrix Renormalization Group: Krylov-space Approach for Correction Vectors
- Quantum Criticality and Spin Liquid Phase in the Shastry-Sutherland model
- Field-induced magnetic transition and spin fluctuation in quantum spin liquid candidate CsYbSe
- Pressure-Tuned Exchange Coupling of a Quantum Spin Liquid in the Molecular Triangular Lattice -(ET)Ag(CN)
- Four-Spin Terms and the Origin of the Chiral Spin Liquid in Mott Insulators on the Triangular Lattice
- Quantum phase diagram of the triangular-lattice antiferromagnet BaCoSbO
- Spectral signatures of fractionalization in the frustrated Heisenberg model on the square lattice
- Gapped magnetic ground state in quantum-spin-liquid candidate -(BEDT-TTF)-Cu(CN)
- Strong quantum interactions prevent quasiparticle decay
- A Class of Compounds Featuring Frustrated Triangular Magnetic Lattice CsRESe (RE=La-Lu): Quantum Spin-Liquid Candidates
- The Spinon Fermi Surface U(1) Spin Liquid in a Spin-Orbit-Coupled Triangular Lattice Mott Insulator YbMgGaO4
- Symmetry fractionalization in the topological phase of the spin- - triangular Heisenberg model
- Hierarchy of exchange interactions in the triangular-lattice spin-liquid YbMgGaO
- Nearest-neighbor resonating valence bonds in YbMgGaO4
- Thermal conductivity of the quantum spin liquid candidate EtMe3Sb[Pd(dmit)2]2: No evidence of mobile gapless excitations
- Site-resolved imaging of ultracold fermions in a triangular-lattice quantum gas microscope
- Fractionalized excitations in the partially magnetized spin liquid candidate YbMgGaO4
- 1/S-expansion study of spin waves in a two-dimensional Heisenberg antiferromagnet
- Spectral functions and time evolution from the Chebyshev recursion
- From spinon band topology to the symmetry quantum numbers of monopoles in Dirac spin liquids
- Anisotropic charge dynamics in the quantum spin-liquid candidate -(BEDT-TTF)Cu(CN)
- Crystalline Electric-Field Excitations in Quantum Spin Liquids Candidate
- Rearrangement of uncorrelated valence bonds evidenced by low-energy spin excitations in YbMgGaO4
- Chiral spin liquid with spinon Fermi surfaces in spin- triangular Heisenberg model
- Phase diagram of the anisotropic triangular lattice Hubbard model
- Survival of itinerant excitations and quantum spin state transitions in YbMgGaO with chemical disorder
- Detecting spin fractionalization in a spinon Fermi surface spin liquid
- Avoided quasiparticle decay and enhanced excitation continuum in the spin-1/2 near-Heisenberg triangular antiferromagnet Ba3CoSb2O9
- Power-law dependence of the optical conductivity observed in the quantum spin-liquid compound κ-(BEDT-TTF)2Cu2(CN)3
- The amplitude mode in three-dimensional dimerized antiferromagnets
- Spin Excitation Spectra of Anisotropic Spin- Triangular Lattice Heisenberg Antiferromagnets
- Quasi-continuous transition from a Fermi liquid to a spin liquid
- Two-spin entanglement distribution near factorized states
- Spinon Fractionalization from Dynamic Structure Factor of Spin-1/2 Heisenberg Antiferromagnet on the Kagome Lattice
- Electron Spin Resonance on the spin-1/2 triangular magnet NaYbS2
- Microscopic phase separation in triangular-lattice quantum spin magnet kappa-(BEDT-TTF)2Cu2(CN)3 probed by muon spin relaxation
- Synthesis and Anisotropic Magnetism in Quantum Spin Liquid Candidates YbSe ( = K and Rb)
- Single-site magnetic anisotropy governed by inter-layer cation charge imbalance in triangular-lattice AYbX
- Monopole Quantum Numbers in the Staggered Flux Spin Liquid
- Velocity of excitations in ordered, disordered and critical antiferromagnets
- Quantum fluctuations in quantum lattice-systems with continuous symmetry
- Superconductivity in the doped quantum spin liquid on the triangular lattice
- Quantum spin liquid phase in the Shastry-Sutherland model detected by an improved level spectroscopic method
- Dynamical properties of the random Heisenberg chain
- Presence and absence of itinerant gapless excitations in the quantum spin liquid candidate EtMeSb[Pd(dmit)]
- Quantum criticality using a superconducting quantum processor
- NMR study of the spin excitations in the frustrated antiferromagnet Yb(BaBO) with a triangular lattice
- Evidence of Two-Spinon Bound States in the Magnetic Spectrum of BaCoSbO
- Theory of the anomalous spin dynamics of spin- triangular lattice Heisenberg antiferromagnet and its application to BaCoSbO
- Disorder-induced broadening of the spin waves in a triangular-lattice quantum-spin-liquid candidate YbZnGaO
- Dynamical spin correlations of the kagome antiferromagnet
- Dynamical response and dimensional crossover for spatially anisotropic antiferromagnets
- Persistent spin dynamics and absence of spin freezing in the - phase diagram of the 2D triangular antiferromagnet YbMgGaO
- NMR relaxation in the spin-1 Heisenberg chain
- Phase coexistence at the first-order Mott-transition revealed by pressure-dependent dielectric spectroscopy of -(BEDT-TTF)Cu(CN)
- Structure Factors of the Kagome-Lattice Heisenberg antiferromagnets at finite temperatures
- Mathematical open problems in Projected Entangled Pair States
- Charge disproportionation in the spin-liquid candidate -(ET)Cu(CN) at 6 K revealed by Cu NQR measurements
- Low-temperature lattice effects in the spin-liquid candidate -(BEDT-TTF)Cu(CN)
- Insights from experiment and calculations into the glass-like transition in the molecular conductor -(BEDT-TTF)Hg(SCN)Cl
- ESR studies on the spin-liquid candidate -(BEDT-TTF)Cu(CN): anomalous response below K
- Field evolution of the spin-liquid candidate YbMgGaO
- A Discrepancy in Thermal Conductivity Measurement Data of Quantum Spin Liquid '-EtMeSb[Pd(dmit)] (dmit = 1,3-Dithiol-2-thione-4,5-dithiolate)
- Persistent spin dynamics in the pressurized spin-liquid candidate YbMgGaO
- Frustrated Quantum Magnetism with Bose Gases in Triangular Optical Lattices at Negative Absolute Temperatures
- Thermal Conductivity in the Triangular-Lattice Antiferromagnet Ba3CoSb2O9
- Resistivity and Thermal Conductivity of an Organic Insulator beta'-EtMe3Sb[Pd(dmit)2]2
- Dynamical spin excitations of topological Haldane gapped phase in the Heisenberg antiferromagnetic chain with single-ion anisotropy
- Phonon-Spectrum Narrowing Induced by Ultrafast Charge Fluctuation in an Organic Dimer Mott Insulator
- Lattice effects in the quasi-two-dimensional valence-bond-solid Mott insulator EtMeP[Pd(dmit)]
- An ARPES Study of the Electronic Structure of the Quantum Spin Liquid EtMe3Sb[Pd(dmit)2]2
Cited by in corpus (31)
- Empowering deep neural quantum states through efficient optimization
- Field-Induced Spin Excitations in the Spin-1/2 Triangular-Lattice Antiferromagnet CsYbSe
- Complete field-induced spectral response of the spin-1/2 triangular-lattice antiferromagnet CsYbSe
- Evidence of Dirac Quantum Spin Liquid in YbZn2GaO5
- Spectral evidence for Dirac spinons in a kagome lattice antiferromagnet
- Dynamical Signatures of Symmetry Broken and Liquid Phases in an Heisenberg Antiferromagnet on the Triangular Lattice
- Quantum Electrodynamics in 2+1 Dimensions as the Organizing Principle of a Triangular Lattice Antiferromagnet
- Spin-Peierls instability of the U(1) Dirac spin liquid
- Phase Diagram of the Easy-Axis Triangular-Lattice Model
- Simulating Spin Dynamics of Supersolid States in a Quantum Ising Magnet
- Evidence of quantum spin liquid state in a Cu-based triangular lattice antiferromagnet
- Superconductivity in doped triangular Mott insulators: the roles of parent spin backgrounds and charge kinetic energy
- Emergent photons and fractionalized excitations in a quantum spin liquid
- Spin dynamics in the Dirac spin liquid YbZnGaO
- Classical dynamics of the antiferromagnetic Heisenberg spin ladder
- Observation of the spiral spin liquid in a triangular-lattice material
- Exciton interacting with a moiré lattice: Polarons, strings, and optical probing of spin correlations
- Modified large- approach to gapless spin liquids, magnetic orders, and dynamics: Application to triangular lattice antiferromagnets
- Prospects for NMR Spectral Prediction on Fault-Tolerant Quantum Computers
- Emergent Quantum Phenomena of Noncentrosymmetric Charge-Density Wave in 1T-Transition Metal Dichalcogenides
- Collective spin oscillations in a magnetized graphene sheet
- Stability of algebraic spin liquids coupled to quantum phonons
- Gapped magnetic ground state in the spin-liquid candidate -(BEDT-TTF)Ag(CN) suggested by magnetic spectroscopy
- Topical review: the nature of the ground state and possibility of a quantum spin liquid in 1T metal dichalcogenides
- Keldysh pseudo-fermion functional renormalization group for quantum magnetism
- Scalable hybrid quantum Monte Carlo simulation of U(1) gauge field coupled to fermions on GPU
- 5d-mediated indirect exchange and effective spin Hamiltonians in Ce triangular-lattice delafossites
- Competing states in the triangular-lattice - Heisenberg model: a dynamical density-matrix renormalization group study
- Unconventional Spin Dynamics and Supersolid Excitations in the Triangular-Lattice XXZ Model
- Quantum spin liquid ground state with the evidence of roton-like excitations at elevated temperatures in the triangular-lattice delafossite YbCuSe
- Fate of Bosonic Topological Edge Modes in the Presence of Many-Body Interactions