Uncovering footprints of dipolar-octupolar quantum spin ice from neutron scattering signatures

Abstract

Recent experiments on Ce${}_2$Zr${}_2$O${}_7$ suggest that this material may host a novel form of quantum spin ice, a three-dimensional quantum spin liquid with an emergent photon. The Ce${}^{3+}$ local moments on the pyrochlore lattice are described by pseudospin 1/2 degrees of freedom, whose components transform as dipolar and octupolar moments under symmetry operations. In principle, there exist four possible quantum spin ice regimes, depending on whether the Ising component is in the dipolar/octupolar channel, and two possible flux configurations of the emergent gauge field. In this work, using exact diagonalization and molecular dynamics, we investigate the equal-time and dynamical spin structure factors in all four quantum spin ice regimes using quantum and classical computations. Contrasting the distinct signatures of quantum and classical results for the four possible quantum spin ice regimes and elucidating the role of quantum fluctuations, we show that the quantum structure factor computed for the $\pi$-flux octupolar quantum spin ice regime is most compatible with the neutron scattering results on Ce${}_2$Zr${}_2$O${}_7$.

arXiv comment6+6 pages, 5+6 figures

References in corpus (34)

• Quantum Spin Liquids
• Quantum Spin Liquid States
• Quantum Spin Liquids
• Pyrochlore Photons: The U(1) Spin Liquid in a S=1/2 Three-Dimensional Frustrated Magnet
• A Field Guide to Spin Liquids
• Quantum Spin Ice: A Search for Gapless Quantum Spin Liquids in Pyrochlore Magnets
• Properties of a classical spin liquid: the Heisenberg pyrochlore antiferromagnet
• Quantum Excitations in Quantum Spin Ice
• The Fascinating World of Landau-Lifshitz-Gilbert Equation: An Overview
• Coulombic Quantum Liquids in Spin-1/2 Pyrochlores
• Seeing the light : experimental signatures of emergent electromagnetism in a quantum spin ice
• Generic quantum spin ice
• Why spin ice obeys the ice rules
• Frustrated quantum rare-earth pyrochlores
• Experimental signatures of a three-dimensional quantum spin liquid in effective spin-1/2 Ce2Zr2O7 pyrochlore
• Quantum spin ices and topological phases from dipolar-octupolar doublets on the pyrochlore lattice
• Quantum Ice : a quantum Monte Carlo study
• Quantum Spin Ice Dynamics in the Dipole-Octupole Pyrochlore Magnet Ce${}_2$Zr${}_2$O${}_7$
• Candidate Quantum Spin Liquid in the Ce\textsuperscript{3+} Pyrochlore Stannate Ce${}_2$Sn${}_2$O${}_7$
• A quantum liquid of magnetic octupoles on the pyrochlore lattice
• Quantum Lattice Model Solver $\mathcal{H}\Phi$
• Symmetry Enriched U(1) Topological Orders for Dipole-Octupole Doublets on a Pyrochlore Lattice
• Dynamical structure factor of the three-dimensional quantum spin liquid candidate NaCaNi${}_2$F${}_7$
• Spin Dynamics in Pyrochlore Heisenberg Antiferromagnets
• The case for a U(1)${}_{\pi }$ Quantum Spin Liquid Ground State in the Dipole-Octupole Pyrochlore Ce${}_2$Zr${}_2$O${}_7$
• Comprehensive study of the dynamics of a classical Kitaev spin liquid
• Sleuthing out exotic quantum spin liquidity in the pyrochlore magnet Ce${}_2$Zr${}_2$O${}_7$
• Quantum spin ice with frustrated transverse exchange: from pi-flux phase to nematic quantum spin liquid
• Quantum spin liquids in the absence of spin-rotation symmetry: application to Herbertsmithite
• The Spectral Periodicity of Spinon Continuum in Quantum Spin Ice
• Pyrochlore U(1) spin liquid of mixed symmetry enrichments in magnetic fields
• Ground state phase diagram of dipolar-octupolar pyrochlores
• Distinguishing dipolar and octupolar quantum spin ices using contrasting magnetostriction signatures
• Competing $U(1)$ and ${\mathbb{Z}}_2$ dipolar-octupolar quantum spin liquids on the pyrochlore lattice: application to Ce${}_2$Zr${}_2$O${}_7$

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• Quantum Spin Ice Response to a Magnetic Field in the Dipole-Octupole Pyrochlore Ce${}_2$Zr${}_2$O${}_7$
• Spectroscopic signatures of fractionalization in octupolar quantum spin ice
• Update of $\mathcal{H}\Phi$: Newly added functions and methods in versions 2 and 3
• $\mu$SR Study of the Dipole-Octupole Quantum Spin Ice Candidate Ce${}_2$Zr${}_2$O${}_7$
• Emergent photons and fractionalized excitations in a quantum spin liquid
• Distinguishing thermodynamics and spectroscopy for octupolar U(1) spin liquid of Ce-pyrochlores
• A pseudofermion functional renormalization group study of dipolar-octupolar pyrochlore magnets
• Finite Temperature Dynamics in 0-Flux and $\pi$-Flux Quantum Spin Ice: Self-Consistent Exclusive Boson Approach
• Dipolar-octupolar correlations and hierarchy of exchange interactions in Ce${}_2$Hf${}_2$O${}_7$
• Two-Peak Heat Capacity Accounts for $R\ln (2)$ Entropy and Ground State Access in the Dipole-Octupole Pyrochlore Ce${}_2$Hf${}_2$O${}_7$
• Classical spin models of the windmill lattice and their relevance for PbCuTe${}_2$O${}_6$
• Single Crystal Diffuse Neutron Scattering Study of the Dipole-Octupole Quantum Spin Ice Candidate Ce${}_2$Zr${}_2$O${}_7$: No Apparent Octupolar Correlations Above $T=0.05$ K
• Magnetic Field Response of Dipolar-Octupolar Quantum Spin Ice
• Towards a global phase diagram of Ce-based dipolar-octupolar pyrochlore magnets under magnetic fields
• Field-induced multipolar character in the dipolar ground state of the honeycomb rare-earth chalcohalide NdOF