Quantum spin torque driven transmutation of antiferromagnetic Mott insulator

Abstract

The standard model of spin-transfer torque (STT) in antiferromagnetic spintronics considers exchange of angular momentum between quantum spins of flowing electrons and noncollinear-to-them localized spins treated as classical vectors. These vectors are assumed to realize Néel order in equilibrium, $\uparrow \downarrow \dots \uparrow \downarrow$, and their STT-driven dynamics is described by the Landau-Lifshitz-Gilbert (LLG) equation. However, many experimentally employed materials (such as archetypal NiO) are strongly electron-correlated antiferromagnetic Mott insulators (AFMI) where localized spins form a ground state quite different from the unentangled Néel state $|\uparrow \downarrow \dots \uparrow \downarrow ⟩$. The true ground state is entangled by quantum spin fluctuations, leading to expectation value of all localized spins being zero, so that LLG dynamics of classical vectors of fixed length rotating due to STT cannot even be initiated. Instead, a fully quantum treatment of both conduction electrons and localized spins is necessary to capture exchange of spin angular momentum between them, denoted as quantum STT. We use a recently developed time-dependent density matrix renormalization group approach to quantum STT to predict how injection of a spin-polarized current pulse into a normal metal layer coupled to AFMI overlayer via exchange interaction and possibly small interlayer hopping -- which mimics, e.g., topological-insulator/NiO bilayer employed experimentally -- will induce nonzero expectation value of AFMI localized spins. This new nonequilibrium phase is a spatially inhomogeneous ferromagnet with zigzag profile of localized spins. The total spin absorbed by AFMI increases with electron-electron repulsion in AFMI, as well as when the two layers do not exchange any charge.

arXiv comment7 pages, 5 figures; Supplemental Material, including a movie, is available from this URL https://wiki.physics.udel.edu/qttg/Publications

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• Spintronics meets density matrix renormalization group: Quantum spin torque driven nonclassical magnetization reversal and dynamical buildup of long-range entanglement
• Quantum many-body states and Green functions of nonequilibrium electron-magnon systems: Localized spin operators vs. their mapping to Holstein-Primakoff bosons
• Topological nature of the proper spin current and the spin-Hall torque
• When can localized spins interacting with conduction electrons in ferro- or antiferromagnets be described classically via the Landau-Lifshitz equation: Transition from quantum many-body entangled to quantum-classical nonequilibrium states
• Fate of entanglement in magnetism under Lindbladian or non-Markovian dynamics and conditions for their transition to Landau-Lifshitz-Gilbert classical dynamics
• Transient dynamics of a magnetic impurity coupled to superconducting electrodes: exact numerics versus perturbation theory
• Electron-mediated entanglement of two distant macroscopic ferromagnets within a nonequilibrium spintronic device
• Effects of the dynamical magnetization state on spin transfer
• Nonclassical dynamics of Néel vector and magnetization accompanied by THz and high-harmonic radiation from ultrafast-light-driven NiO antiferromagnet insulator
• Geometrical torque on magnetic moments coupled to a correlated antiferromagnet