Ab initio calculation of the electron capture spectrum of 163Ho: Auger-Meitner decay into continuum states
arXiv:2002.05989 · doi:10.1088/1367-2630/abac72
Abstract
Determining the electron neutrino mass by electron capture in Ho relies on an accurate understanding of the differential electron capture nuclear decay rate as a function of the distribution of the total decay energy between the neutrino and electronic excitations. The resulting spectrum is dominated by resonances due to local atomic multiplet states with core holes. Coulomb scattering between electrons couple the discrete atomic states, via Auger-Meitner decay, to final states with free electrons. The atomic multiplets are above the auto-ionisation energy, such that the delta functions representing these discrete levels turn into a superposition of Lorentzian, Mahan- and Fano-like line-shapes. We present an \textit{ab initio} method to calculate nuclear decay modifications due to such processes. It includes states with multiple correlated holes in local atomic orbitals interacting with unbound Auger-Meitner electrons. A strong energy-dependent, asymmetric broadening of the resonances in good agreement with recent experiments is found. We present a detailed analysis of the mechanisms determining the final spectral line-shape and discuss both the Fano interference between different resonances, as well as the energy dependence of the Auger-Meitner Coulomb matrix elements. The latter mechanism is shown to be the dominant channel responsible for the asymmetric line-shape of the resonances in the electron capture spectrum of Ho.
References in corpus (17)
- An improved upper limit on the neutrino mass from a direct kinematic method by KATRIN
- Multiplet ligand-field theory using Wannier orbitals
- HOLMES - The Electron Capture Decay of 163Ho to Measure the Electron Neutrino Mass with sub-eV sensitivity
- Direct Measurement of the Mass Difference of Ho163 and Dy163 Solves the Q-Value Puzzle for the Neutrino Mass Determination
- Bands, resonances, edge singularities and excitons in core level spectroscopy investigated within the dynamical mean field theory
- Development of holmium-163 electron-capture spectroscopy with transition-edge sensors
- Examination of the calorimetric spectrum to determine the neutrino mass in low-energy electron capture decay
- Search for Oscillation of the Electron-Capture Decay Probability of Pm
- Improved Description of One- and Two-Hole States after Electron Capture in 163 Holmium and the Determination of the Neutrino Mass
- Determination of the neutrino mass by electron capture in 163 Holmium and the role of the three-hole states in 163 Dysprosium
- Neutrino Mass, Electron Capture and the Shake-off Contributions
- The calorimetric spectrum of the electron-capture decay of Ho. The spectral endpoint region
- calculation of the calorimetric electron capture spectrum of Holmium: Intra-atomic decay into bound-states
- Measurement of the intensity ratio of Auger and conversion electrons for the electron capture decay of I
- High-resolution conversion electron spectroscopy of the 125I electron-capture decay
- Search for environmental effects on the KLL Auger spectrum of rubidium generated in radioactive decay
- First Calorimetric Measurement of Electron Capture in Pt with a Transition Edge Sensor
Cited by in corpus (10)
- Direct Measurements of Neutrino Mass
- Dy electron-capture: a strong new candidate for neutrino mass determination
- High-precision electron-capture value measurement of In for electron-neutrino mass determination
- Most stringent bound on electron neutrino mass obtained with a scalable low temperature microcalorimeter array
- Metallic magnetic calorimeter arrays for the first phase of the ECHo experiment
- Neutrino mass measurements using cryogenic detectors
- Development and characterisation of high-resolution microcalorimeter detectors for the ECHo-100k experiment
- New targets for relic antineutrino capture
- Phenomenological Modeling of the Ho Calorimetric Electron Capture Spectrum from the HOLMES Experiment
- Data reduction for a calorimetrically measured spectrum of the ECHo-1k experiment