Thermoelectric conversion at 30K in InAs/InP nanowire quantum dots
arXiv:1903.06935 · doi:10.1021/acs.nanolett.9b00276
Abstract
We demonstrate high-temperature thermoelectric conversion in InAs/InP nanowire quantum dots by taking advantage of their strong electronic confinement. The electrical conductance G and the thermopower S are obtained from charge transport measurements and accurately reproduced with a theoretical model accounting for the multi-level structure of the quantum dot. Notably, our analysis does not rely on the estimate of co-tunnelling contributions since electronic thermal transport is dominated by multi-level heat transport. By taking into account two spin-degenerate energy levels we are able to evaluate the electronic thermal conductance K and investigate the evolution of the electronic figure of merit ZT as a function of the quantum dot configuration and demonstrate ZT ~ 35 at 30 K, corresponding to an electronic effciency at maximum power close to the Curzon- Ahlborn limit.
arXiv comment7 pages, 4 figures
References in corpus (47)
- A single-atom heat engine
- Fundamental aspects of steady-state conversion of heat to work at the nanoscale
- Thermoelectric energy harvesting with quantum dots
- Thermoelectric efficiency at maximum power in a quantum dot
- A quantum-dot heat engine operating close to the thermodynamic efficiency limits
- Optimal energy quanta to current conversion
- Thermopower of Single-Molecule Devices
- Thermoelectric transport through strongly correlated quantum dots
- Optimal thermoelectric figure of merit of a molecular junction
- Violation of the Wiedemann-Franz Law in a Single-Electron Transistor
- Large enhancement of thermoelectric effects in a double quantum dot system due to interference and Coulomb correlation phenomena
- Thermoelectric efficiency at maximum power in low-dimensional systems
- Increasing thermoelectric performance using coherent transport
- Three-terminal thermoelectric transport through a molecular junction
- Powerful and efficient energy harvester with resonant-tunneling quantum dots
- Cotunneling thermopower of single electron transistors
- Thermoelectric effects in Kondo correlated quantum dots
- Nonlinear thermovoltage and thermocurrent in quantum dots
- Thermal and Thermoelectric Transport in Nanostructures and Low-Dimensional Systems
- Thermoelectric efficiency of three-terminal quantum thermal machines
- Three-terminal thermoelectric transport through a molecule placed on an Aharonov-Bohm ring
- Nonlinear heat transport in mesoscopic conductors: Rectification, Peltier effect and Wiedemann-Franz law
- Spin-thermopower in interacting quantum dots
- Sequential and co-tunneling behavior in the temperature-dependent thermopower of few-electron quantum dots
- Thermal Conductance of a Single-Electron Transistor
- Thermoelectric properties of an interacting quantum dot-based heat engine
- Lineshape of the thermopower of quantum dots
- Direct measurement of the Seebeck coefficient in a Kondo-correlated single-quantum-dot transistor
- Strongly nonlinear thermovoltage and heat dissipation in interacting quantum dots
- Absorption refrigerators based on Coulomb-coupled single-electron systems
- Quantum-fluctuation effects on the thermopower of a single-electron transistor
- Measuring Temperature Gradients over Nanometer Length Scales
- Coulomb Blockade Oscillations in the Thermopower of Open Quantum Dots
- Nanoscale spin rectifiers controlled by the Stark effect
- Manipulation of electron orbitals in hard-wall InAs/InP nanowire quantum dots
- ThermoElectric Transport Properties of a Chain of Quantum Dots with Self-Consistent Reservoirs
- Reversible electron-hole separation in a hot carrier solar cell
- Thermal drag in electronic conductors
- Experimental realization of a Coulomb blockade refrigerator
- The interacting resonant level model in nonequilibrium: finite temperature effects
- The effect of Coulomb interactions on nonlinear thermovoltage and thermocurrent in quantum dots
- Single-nanowire, low-bandgap hot carrier solar cells with tunable open-circuit voltage
- Nonlinear thermoelectric response due to energy-dependent transport properties of a quantum dot
- Quantum-dot thermometry
- Signatures of exchange correlations in the thermopower of quantum dots
- Thermoelectric spin accumulation and long-time spin precession in a non-collinear quantum dot spin valve
- Strongly-Correlated Thermoelectric Transport beyond Linear Response
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- Superconducting Spintronic Heat Engine
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