Micro-engineered CH${}_3$NH${}_3$PbI${}_3$ nanowire/graphene phototransistor for low intensity light detection at room temperature

Abstract

Methylammonium lead iodide perovskite has revolutionized the field of third generation solid-state solar cells leading to simple solar cell structures1 and certified efficiencies up to 20.1%. Recently the peculiar light harvesting properties of organometal halide perovskites have been exploited in photodetectors where responsivities of ~3.5 A/W and 180 A/W have been respectively achieved for pure perovskite-based devices and hybrid nanostructures. Here, we report on the first hybrid phototransistors where the performance of a network of photoactive Methylammonium Lead Iodide nanowires (hereafter MAPbI${}_3$NW) are enhanced by CVD-grown monolayer graphene. These devices show responsivities as high as ~2.6x10${}^6$ A/W in the visible range showing potential as room-temperature single-electron detector.

References in corpus (2)

• Detection of Individual Gas Molecules Absorbed on Graphene
• Intrinsic Response of Graphene Vapor Sensors

Cited by in corpus (6)

• Ultrasensitive 3D Aerosol-Jet-Printed Perovskite X-Ray Photodetector
• Controlled growth of CH${}_3$NH${}_3$PbI${}_3$ nanowires in arrays of open nanofluidic channels
• Light-Emitting Electrochemical Cells of Single Crystal Hybrid Halide Perovskite with Vertically Aligned Carbon Nanotubes Contacts
• Ultrasensitive 1D field-effect phototransistor: CH${}_3$NH${}_3$PbI${}_3$ nanowire sensitized individual carbon nanotube
• Three-dimensionally Enlarged Photoelectrodes by a Protogenetic Inclusion of Vertically Aligned Carbon Nanotubes into CH3NH3PbBr3 Single Crystals
• Influence of the organic cation disorder on photoconductivity in ethylenediammonium lead iodide, NH3CH2CH2NH3PbI4