paper

Microscopic view on the ultrafast photoluminescence from photo-excited graphene

arXiv:1411.0531 · doi:10.1021/nl504176z

Abstract

We present a joint theory-experiment study on ultrafast photoluminescence from photoexcited graphene. Based on a microscopic theory, we reveal two distinct mechanisms behind the occurring photoluminescence: Besides the well-known incoherent contribution driven by non-equilibrium carrier occupations, we found a coherent part that spectrally shifts with the excitation energy. In our experiments, we demonstrate for the first time the predicted appearance and spectral shift of the coherent photoluminescence.

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