A new regime of nanoscale thermal transport: collective diffusion counteracts dissipation inefficiency
arXiv:1407.0658 · doi:10.1073/pnas.1503449112
Abstract
Understanding thermal transport from nanoscale heat sources is important for a fundamental description of energy flow in materials, as well as for many technological applications including thermal management in nanoelectronics, thermoelectric devices, nano-enhanced photovoltaics and nanoparticle-mediated thermal therapies. Thermal transport at the nanoscale is fundamentally different from that at the macroscale and is determined by the distribution of carrier mean free paths in a material, the length scales of the heat sources, and the distance over which heat is transported. Past work has shown that Fourier's law for heat conduction dramatically over-predicts the rate of heat dissipation from heat sources with dimensions smaller than the mean free path of the dominant heat-carrying phonons. In this work, we uncover a new regime of nanoscale thermal transport that dominates when the separation between nanoscale heat sources is small compared with the dominant phonon mean free paths. Surprisingly, the interplay between neighboring heat sources can facilitate efficient, diffusive-like heat dissipation, even from the smallest nanoscale heat sources. This finding suggests that thermal management in nanoscale systems including integrated circuits might not be as challenging as projected. Finally, we demonstrate a unique and new capability to extract mean free path distributions of phonons in materials, allowing the first experimental validation of differential conductivity predictions from first-principles calculations.
arXiv commentMain text: 18 pages, 4 figures. Supplementary Information: 13 pages, 9 figures
References in corpus (8)
- Bright Coherent Ultrahigh Harmonics in the keV X-Ray Regime from Mid-Infrared Femtosecond Lasers
- Phase-Matched Generation of Coherent Soft-X-Rays
- Direct Measurement of Room Temperature Non-diffusive Thermal Transport Over Micron Distances in a Silicon Membrane
- Anomalous Heat Diffusion
- Anomalous Heat Diffusion
- Anomalous Heat Conduction and Anomalous Diffusion in Low Dimensional Nanoscale Systems
- Onset of non-diffusive phonon transport in transient thermal grating decay
- Ab-initio calculation of all-optical time-resolved calorimetry of nanosized systems: Evidence of nanosecond-decoupling of electron and phonon temperatures
Cited by in corpus (41)
- Measurement Techniques for Thermal Conductivity and Interfacial Thermal Conductance of Bulk and Thin Film Materials
- Tutorial: Time-domain thermoreflectance (TDTR) for thermal property characterization of bulk and thin film materials
- Non-Destructive, High-Resolution, Chemically Specific, 3D Nanostructure Characterization using Phase-Sensitive EUV Imaging Reflectometry
- Thermal Transport in 3D Nanostructures
- Machine Learning for Predicting Thermal Transport Properties of Solids
- Ptychographic hyperspectral spectromicroscopy with an extreme ultraviolet high harmonic comb
- Nanoscale diffractive probing of strain dynamics in ultrafast transmission electron microscopy
- First principles Kinetic-Collective thermal conductivity of semiconductors
- Lagging Heat Models in Thermodynamics and Bioheat Transfer: a Critical Review
- Non-Fourier heat transport in nanosystems
- Temperonic Crystal: a superlattice for temperature waves in graphene
- Thermal transport from 1D- and 2D-confined nanostructures on silicon probed using coherent extreme UV light: General and predictive model yields new understanding
- Accessing temperature waves: a dispersion relation perspective
- Crossover from ballistic to normal heat transport in the lattice: If nonconservation of momentum is the reason, what is the mechanism?
- Ultrahigh convergent thermal conductivity of carbon nanotubes from comprehensive atomistic modeling
- Steady State and Modulated Heat Conduction in Layered Systems Predicted by the Phonon Boltzmann Transport Equation
- Monte Carlo Study of Non-diffusive Relaxation of A Transient Thermal Grating in Thin Membranes
- MCBTE: A variance-reduced Monte Carlo solution of the linearized Boltzmann transport equation for phonons
- A numerical ellipsometric analysis (NEA) of nanoscale layered systems
- Universal behavior of highly-confined heat flow in semiconductor nanosystems: from nanomeshes to metalattices
- Heat dissipation in the quasiballistic regime studied using Boltzmann equation in the spatial frequency domain
- A Variational Approach to Extracting the Phonon Mean Free Path Distribution from the Spectral Boltzmann Transport Equation
- Thermal boundary resistance from transient nanocalorimetry: a multiscale modeling approach
- Effective thermal conductivity of rectangular nanowires based on phonon hydrodynamics
- Variational Approach to Solving the Spectral Boltzmann Transport Equation in Transient Thermal Grating for Thin Films
- Thermal dynamics and electronic temperature waves in layered correlated materials
- Quasiballistic heat removal from small sources studied from first principles
- Analysis of nonlocal phonon thermal conductivity simulations showing the ballistic to diffusive crossover
- Modeling quasi-ballistic transient thermal transport with spatially sinusoidal heating: a McKelvey-Shockley flux approach
- Ultrafast X-ray Diffraction Thermometry Measures the Influence of Spin Excitations on the Heat Transport through nanolayers
- Ab Initio Modeling of Thermal Transport through van der Waals Materials
- Compact models for multidimensional quasiballistic thermal transport
- Monte Carlo Simulation of Single-Crystalline PbSe Nanowire Thermal Conductivity Using First-Principle Phonon Properties
- Heat Transport with a Twist
- Non-monotonic heat dissipation phenomenon in close-packed quasi-2D and 3D hotspot system
- Shear Forces and Heat Conductance in Nanoscale Junctions
- Descriptors of intrinsic hydrodynamic thermal transport: screening a phonon database in a machine learning approach
- Relativistic stable processes in quasi-ballistic heat conduction in thin film semiconductors
- Non-local thermal transport modeling using the thermal distributor
- Transient microscopy for measuring heat transfer in single cells
- Energy relaxation and thermal diffusion in IR pump-probe spectroscopy of hydrogen-bonded liquids